High-speed antiferromagnetic domain walls driven by coherent spin waves

TL;DR

This paper demonstrates ultrafast control of antiferromagnetic domain walls using coherent spin waves generated by ultrafast laser pulses, achieving record-high velocities and bidirectional control, advancing high-speed spintronic applications.

Contribution

It experimentally realizes coherent spin wave-driven AFM domain wall motion at record speeds and introduces a controllable, bidirectional propulsion mechanism in an easy-plane AFM insulator.

Findings

AFM domain walls reach velocities up to 50 km/s.

DW propagation direction is controllable via laser helicity and winding number.

The mechanism is explained by in-plane magnon mode dynamics.

Abstract

The ability to rapidly manipulate domain walls (DWs) in magnetic materials is key to developing novel high-speed spintronic memory and computing devices. Antiferromagnetic (AFM) materials present a particularly promising platform due to their robustness against stray fields and their potential for exceptional DW velocities. Among various proposed driving mechanisms, coherent spin waves could potentially propel AFM DWs to the magnon group velocity while minimizing dissipation from Joule heating. However, experimental realization has remained elusive due to the dual challenges of generating coherent AFM spin waves near isolated mobile AFM DWs and simultaneously measuring high-speed DW dynamics. Here we experimentally realize an approach where ultrafast laser pulses generate coherent spin waves that drive AFM DWs and develop a technique to directly map the spatiotemporal DW dynamics. Using the room-temperature AFM insulator Sr$_2$Cu$_3$O$_4$Cl$_2$, we observe AFM DW motion with record-high velocities up to ~50 km/s. Remarkably, the direction of DW propagation is controllable through both the pump laser helicity and the sign of the DW winding number. This bidirectional control can be theoretically explained, and numerically reproduced, by the DW dynamics induced by coherent spin waves of the in-plane magnon mode - a phenomenon unique to magnets with an easy-plane anisotropy. Our work uncovers a novel DW propulsion mechanism that is generalizable to a wide range of AFM materials, unlocking new opportunities for ultrafast coherent AFM spintronics.