Aging in the Flow Dynamics of Dense Suspensions of Contactless Microparticles

TL;DR

This paper investigates how the flow behavior of dense contactless microparticle suspensions depends on resting time, revealing aging effects that influence flow onset and velocity, with implications for understanding intermediate states between colloids and granular media.

Contribution

It demonstrates that aging effects in dense microparticle suspensions depend on resting time and are reversible, highlighting a new form of aging between colloidal and granular behaviors.

Findings

Longer resting times delay flow onset and reduce velocity.

Aging effects are reversible with agitation, restoring initial flow properties.

Aging occurs without changes in packing fraction, in both monodisperse and polydisperse piles.

Abstract

This study demonstrates that the free-surface flow dynamics of dense piles of contactless silica microparticles depend on the resting period prior to flow. Microfluidic rotating drum experiments reveal that longer resting times lead to delayed flow onsets and reduced flow velocities, both evolving logarithmically with the resting time. These aging-like effects are more pronounced for thermally driven creep flows in piles with initial tilting angle below the athermal angle of repose, in contrast to piles initially tilted above this repose angle, where gravity-driven flows tend to gradually erase aging effects. Moreover, we show that the packing fraction does not change during the resting period, and that aging occurs in both monodisperse and polydisperse piles, indicating that crystallization is not required for the time-dependent behavior to appear. Remarkably, vigorous agitation that re-disperses the particles fully restores the piles to their initial state, demonstrating that the observed effects are not due to sample degradation. These findings evidence a form of aging in quiescent suspensions intermediate between colloidal and granular media, where thermal fluctuations, still significant relative to particle weight, progressively stabilize the system, making it more resistant to flow and deformation.