# Toward triggered generation of indistinguishable single-photons from MoTe$_2$ quantum emitters

**Authors:** Pawe{\l} Wyborski, Athanasios Paralikis, Pietro Metuh, Martin A. Jacobsen, Christian Ruiz, Niels Gregersen, Battulga Munkhbat

arXiv: 2508.20743 · 2025-08-29

## TL;DR

This paper demonstrates near-infrared single-photon emitters in bilayer MoTe2 with high purity, tunability, and the highest reported indistinguishability for TMD quantum emitters, advancing telecom-compatible quantum photonics.

## Contribution

It introduces a reproducible method for creating tunable, high-quality single-photon sources in MoTe2 with record-high indistinguishability in the near-infrared.

## Key findings

- Emitters show >70% linear polarization and sub-450 ps lifetimes.
- Electrostatic biasing achieves 3 meV Stark tuning and reduces linewidths.
- Two-photon interference visibility reaches 40% with filtering.

## Abstract

Single-photon sources operating in the telecom band are fundamental components for long-distance optical quantum communication and information processing. Two-dimensional (2D) transition metal dichalcogenides (TMDs) offer a promising platform for such sources, but their development has been hindered by limited spectral range and poor single-photon indistinguishability. Here, we demonstrate a reproducible and systematic approach for generating near-infrared (1090-1200 nm) quantum emitters in bilayer MoTe$_2$ using deterministic strain and defect engineering. These emitters exhibit strong linear polarization (DOLP $>70\%$), sub-nanosecond lifetimes ($\tau \leqslant$ ~450 ps), high single-photon purity ($g^{(2)}(0)<0.1$), and resolution-limited emission ($\sim$200 $\mu$eV). Electrostatic biasing enables Stark tuning over a $\sim$3 meV range, reduced photon bunching, and significantly shortened radiative lifetimes, yielding narrow emission with ratios of experimental to transform-limited linewidths as low as $R\sim55$. Most notably, two-photon interference measurements reveal a Hong-Ou-Mandel visibility of $V_\text{HOM}\sim $10$\%$, and up to $V_\text{HOM}\sim$ 40$\%$ with post-selection by temporal filtering, representing the highest reported indistinguishability for any TMD quantum emitters and the first such demonstration in the near-infrared regime. These results establish MoTe$_2$ as a viable platform for tunable, low-noise, high-purity single-photon sources with promising indistinguishability, paving the way for their integration into telecom-compatible quantum photonic technologies.

## Full text

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## Figures

5 figures with captions in the complete paper: https://tomesphere.com/paper/2508.20743/full.md

## References

61 references — full list in the complete paper: https://tomesphere.com/paper/2508.20743/full.md

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Source: https://tomesphere.com/paper/2508.20743