Disorder-induced stress-flow misalignment in soft glassy materials revealed using multi-directional shear

TL;DR

This study reveals how complex shear histories induce anisotropic stress responses in soft glassy materials, highlighting the role of internal disorder and providing new insights into their mechanical behavior under multi-directional shear.

Contribution

It introduces a multi-axis shear apparatus and demonstrates how shear history causes stress-flow misalignment and anisotropic yield surfaces in soft glassy materials.

Findings

Transient shear response orthogonal to applied shear direction

Anisotropic yield surface observed in experiments

Internal stress distribution imprinted by deformation

Abstract

Controlling the mechanical response of soft glassy materials, such as emulsions, foams, and colloidal suspensions, is key for many industrial processes. While their steady-state flow behavior is reasonably well understood, their response to complex flow histories, as encountered in operations like pumping or mixing, remains poorly known. Using a custom multi-axis shear apparatus that enables arbitrary changes in flow direction, we investigate how shear history influences the mechanical behavior of a model soft glassy system. We uncover a transient shear response orthogonal to the applied shear direction, together with an anisotropic yield surface. These effects point to an underlying anisotropic distribution of internal stresses imprinted by previous deformation. To rationalize this behavior, we use a mesoscopic elasto-plastic model, demonstrating that local mechanical disorder governs the emergence of macroscopic stress-flow misalignment. Our findings offer a new route to experimentally probe the distribution of local yield stresses in soft glassy materials.