Beyond fragmented dopant dynamics in quantum spin lattices: Robust localization and non-Gaussian diffusion

TL;DR

This paper explores dopant dynamics in quantum spin lattices, revealing robust localization at nonzero temperatures and non-Gaussian diffusion behavior, with implications for understanding high-temperature superconductivity.

Contribution

It demonstrates that dopants are localized in Ising limit due to emergent disordered potentials and uncovers non-monotonic diffusion dependence on spin-exchange rate using advanced matrix-product-state calculations.

Findings

Dopants are localized at nonzero temperatures in Ising limit.

Diffusion coefficient depends non-monotonically on spin-exchange rate.

Diffusion exhibits self-similar, non-Gaussian scaling behavior.

Abstract

The motion of dopants in magnetic spin lattices has received tremendous attention for at least four decades due to its connection to high-temperature superconductivity. Despite these efforts, we lack a complete understanding of their behavior, especially out of the equilibrium and at nonzero temperatures. In this paper, we take a significant step towards a much deeper understanding based on state-of-the-art matrix-product-state calculations. In particular, we investigate the non-equilibrium dynamics of a dopant in two-leg $t$--$J$ ladders with antiferromagnetic XXZ spin interactions. In the Ising limit, we find that the dopant is localized for all investigated nonzero temperatures due to an emergent disordered potential, with a localization length controlled by the underlying correlation length of the spin lattice, which increases exponentially with decreasing temperature. The dopant, hereby, only delocalizes asymptotically in the zero temperature limit. This greatly generalizes the localization effect discovered recently in Hilbert space fragmented models. In the presence of spin-exchange processes at rate $\alpha$, the dopant diffuses with a diffusion coefficient, $D_h$, depending non-monotonically on $\alpha$. It initially increases linearly as $D_h \propto \alpha$ for $\alpha \ll 1$ before dropping off as $\alpha^{-1}$ for $\alpha > 1$. Moreover, we show that the underlying spin dynamics at infinite temperature behaves qualitatively the same, albeit with important quantitative differences. We substantiate these findings by showing that the dynamics features self-similar scaling behavior, which strongly deviates from the Gaussian behavior of regular diffusion, especially for weak spin exchange. Finally, we show that the diffusion coefficient $D_h$ follows an Arrhenius relation at high temperatures, whereby it is exponentially suppressed upon cooling.