Spin-orbit crossover and the origin of magnetic torque in kagome metals

TL;DR

This paper proposes a novel interband spin-orbit coupling mechanism to explain the nematic magnetic torque and related phenomena observed in kagome metal CsV$_3$Sb$_5$, challenging previous charge density wave explanations.

Contribution

It introduces a new interband ordering framework involving spin-orbit coupling and symmetry-breaking, providing a comprehensive explanation for the observed magnetic torque features.

Findings

The theory explains the onset of magnetic torque at T_τ as a crossover in interband spin-orbit coupling.

It accounts for hysteresis and the absence of nematicity in elastoresistance measurements.

Predicts strain-induced magnetization as a testable consequence.

Abstract

Recent experiments on the kagome metal CsV$_3$Sb$_5$ reveal a curious phase transition-like feature: a nematic magnetic torque response that abruptly sets in at $T_\tau \approx 130$K, above the known charge density wave transition at $T_\text{CDW} \approx 100$K. Counterintuitively, elastoresistance measurements--a standard probe of nematicity--show no corresponding signal, ruling out a nematic phase transition and placing strong constraints on possible explanations. Beyond nematicity, the torque is paramagnetic for in-plane magnetic field, while above a critical out-of-plane field, an in-plane magnetisation appears, accompanied by hysteresis. We show that this combination of features cannot be accounted for by charge density waves or intraband magnetic order. Instead, we propose that interband ordering--via a symmetry-allowed interband spin-orbit coupling and a time-reversal and spatial symmetry-breaking interband order parameter--together with a background strain field, consistent with typical experimental conditions, provides a natural explanation; in our picture, the behaviour at $T_\tau$ is understood as a crossover in the symmetry-allowed interband spin-orbit coupling strength. Our theory accounts for the nematic magnetic torque, hysteresis, and the transition-like onset at $T_\tau$, while also making testable predictions, including strain-induced magnetisation. In doing so, it challenges the prevailing view of the normal state.