Optimization and characterization of laser excitation for quantum sensing with single nitrogen-vacancy centres

TL;DR

This paper presents a comprehensive method for characterizing and optimizing laser excitation parameters in confocal microscopy to improve quantum sensing with single nitrogen-vacancy centers, ensuring reliable and enhanced sensor performance.

Contribution

It introduces a systematic protocol for optimizing laser parameters in NV center experiments, improving the reliability and effectiveness of quantum sensing applications.

Findings

Optimized laser beam profile and polarization for NV centers.

Confirmed single-emitter operation via $g^{(2)}(\tau)$ measurement.

Demonstrated improved control of spin transitions in NV centers.

Abstract

In this work we present a comprehensive method of characterization and optimization of laser irradiation within a confocal microscope tailored to quantum sensing experiments using nitrogen-vacancy (NV) centres. While confocal microscopy is well-suited for such experiments, precise control and understanding of several optical parameters are essential for reliable single-emitter studies. We investigate the laser beam intensity profile, single-photon emission statistics, fluorescence response under varying polarization and saturation conditions, spectral characteristics, and the temporal profiles of readout and reinitialization pulses. The beam quality is assessed using the beam propagation factor $M^2$, determined via the razorblade technique. Optical fluorescence spectrum is recorded to confirm NV centre emission. To confirm single-emitter operation, we measure second-order autocorrelation function $g^{(2)}(\tau)$. Saturation behaviour is analysed by varying laser power and recording the corresponding fluorescence, while polarization dependence is studied using a half-wave ($\lambda/2$) plate. Temporal laser pulse profile is examined by modulating the power of an acousto-optic modulator. After optimizing all relevant parameters, we demonstrate the microscope's capabilities in driving spin transitions of a single NV centre. This work establishes a straightforward and effective protocol for laser excitation optimization, enhancing the performance and reliability of NV-based quantum sensors.