Time-resolved three-dimensional elucidation of complex-refractive-index alteration induced by ultrashort laser pulses

TL;DR

This paper introduces a novel polarization-based method for three-dimensional, time-resolved mapping of complex refractive index changes caused by ultrashort laser pulses, advancing understanding of laser-matter interactions.

Contribution

It presents the first accurate 3D measurement technique for ultrafast complex refractive index fluctuations induced by ultrashort laser pulses.

Findings

First 3D mapping of ultrafast refractive index changes

Provides insights into ablation mechanisms

Enhances understanding of laser-induced material modifications

Abstract

Ultrashort pulse lasers (USPLs) have attracted attention as tools capable of inducing unique phenomena by instantaneously generating regions with transiently modified properties (filaments) in the material. However, a comprehensive understanding of USPL-induced filaments remains elusive due to the complexity of their dynamics and insufficient imaging techniques to accurately capture them. In this study, we propose a novel methodology to measure the transient complex refractive index of filaments through polarization analysis of a probe pulse. To our knowledge, this approach achieves, for the first time, accurate three dimensional mapping of the ultrafast fluctuations in complex refractive index. The present findings provide critical insights into the ablation mechanisms driven by USPLs, essential for optimizing laser parameters in micro- and nanoprocessing. Moreover, this work contributes valuable experimental data to condensed matter and computational physics by elucidating the physical properties of USPL-irradiated regions.