Spin-Photon Correlations from a Purcell-enhanced Diamond Nitrogen-Vacancy Center Coupled to an Open Microcavity

TL;DR

This paper demonstrates a highly efficient spin-photon interface using a Purcell-enhanced diamond nitrogen-vacancy center coupled to an open microcavity, enabling improved quantum state control and entanglement generation.

Contribution

It introduces a novel microcavity design achieving significant Purcell enhancement and efficient spin-photon coupling in diamond NV centers.

Findings

Purcell factor of 7.3 ± 1.6 achieved

Photon detection probability of 0.5% per pulse

Generation of two- and three-qubit spin-photon states

Abstract

An efficient interface between a spin qubit and single photons is a key enabling system for quantum science and technology. We report on a coherently controlled diamond nitrogen-vacancy center electron spin qubit that is optically interfaced with an open microcavity. Through Purcell enhancement and an asymmetric cavity design, we achieve efficient collection of resonant photons, while on-chip microwave lines allow for spin qubit control at a 10 MHz Rabi frequency. With the microcavity tuned to resonance with the nitrogen-vacancy center's optical transition, we use excited state lifetime measurements to determine a Purcell factor of 7.3 $\pm$ 1.6. Upon pulsed resonant excitation, we find a coherent photon detection probability of 0.5 % per pulse. Although this result is limited by the finite excitation probability, it already presents an order of magnitude improvement over the solid immersion lens devices used in previous quantum network demonstrations. Furthermore, we use resonant optical pulses to initialize and read out the electron spin. By combining the efficient interface with spin qubit control, we generate two-qubit and three-qubit spin-photon states and measure heralded Z-basis correlations between the photonic time-bin qubits and the spin qubit.