Excitations and dynamical structure factor of $J_1-J_2$ spin-$3/2$ and spin-$5/2$ Heisenberg spin chains

TL;DR

This paper investigates the dynamical structure factor of frustrated spin-$3/2$ and spin-$5/2$ Heisenberg chains, revealing incommensurate excitations, complex spectral features, and the universality of fractionalization phenomena across higher spins.

Contribution

It introduces a combined valence bond solid and DMRG approach to analyze incommensurate excitations and spectral features in higher-spin frustrated chains, highlighting universal behaviors.

Findings

Magnon develops incommensurate dispersion at J2 ≈ 0.32J1.

Spinons become incommensurate at J2 ≈ 0.4J1, beyond the Lifshitz point.

Spinon gap exhibits nonmonotonic behavior, indicating a floating phase.

Abstract

We study the dynamical structure factor of the frustrated spin-$3/2$ $J_1$-$J_2$ Heisenberg chains, with particular focus on the partially dimerized phase that emerges between two Kosterlitz-Thouless transitions. Using a valence bond solid ansatz corroborated by density matrix renormalization group simulations, we investigate the nature of magnon and spinon excitations through the single-mode approximation. We show that the magnon develops an incommensurate dispersion at $J_2 \approx 0.32J_1$, while the spinons, viewed as domain walls between degenerate valence bond solid states, become incommensurate at $J_2 \approx 0.4J_1$ beyond the Lifshitz point ($J_2 \approx 0.388J_1$). The dynamical structure factor exhibits rich spectral features shaped by the interplay between these excitations, with magnons appearing as resonances embedded in the spinon continuum. The spinon gap shows a nonmonotonic behavior, reaching a peak near the center of the partially dimerized phase and closing at the boundaries, suggesting the appearance of a floating phase as a result of the condensation of incommensurate spinons. Comparative analysis with the spin-$5/2$ case confirms the universality of these phenomena across half-integer higher-spin systems. Our results provide detailed insight into how fractionalization and incommensurate condensation govern the spectral properties of frustrated spin chains, offering a unified picture across different spin magnitudes.