Dynamic Control of Momentum-Polarization Photoluminescence States with Liquid-Crystal-tuned Nanocavities

TL;DR

This paper presents a liquid-crystal-tuned nanocavity device that dynamically controls the directionality and polarization of photoluminescence from perovskite materials, enabling advanced beam steering with high tunability.

Contribution

Introduction of a novel liquid-crystal-tunable Fabry-Perot nanocavity that allows continuous, electrical control of emission angle and polarization of photoluminescence from perovskites.

Findings

Achieved emission angle tuning up to 28 degrees.

Demonstrated polarization manipulation and conversion.

Observed a threefold increase in emission intensity.

Abstract

Dynamic control of light, and in particular beam steering, is pivotal in various optical applications, including telecommunications, LiDAR, and biomedical imaging. Traditional approaches achieve this by interfacing a tunable modulating device with an external light source, facing challenges in achieving compact devices. Here, we introduce a dynamic photoluminescence (PL) modulating device, with which the properties of light directly emitted by a quasi-two-dimensional perovskite (in particular its directionality and polarization) can be modified continuously and over a large range. The device is based on a liquid-crystal-tunable Fabry-Perot (FP) nanocavity and uses the FP energy-momentum dispersion and spin-orbit coupling between the excitons and the cavity modes to enable this dynamic control over the emitted radiation. With this device, we achieve electrically-controlled, continuous and variable emission angles up to a maximum of 28{\deg}, as well as manipulation of the PL polarization state, enabling both the creation of polarization gradients and the achievement of polarization conversion at specific emission angles. Moreover, due to its resonant character, a 3-fold increase in the emission intensity is observed, as confirmed through time-resolved photoluminescence (TRPL) measurements. Our approach leverages the unique properties of actively tunable birefringent nanocavities to improve emission directivity, angle tunability and polarization control, presenting a promising solution for next-generation, deeply integrated beam steering devices.