Quantum engineering of high harmonic generation
Neda Boroumand, Adam Thorpe, Graeme Bart, Lu Wang, David N. Purschke, Giulio Vampa, Thomas Brabec

TL;DR
This paper develops a theoretical framework for quantum sideband high harmonic generation, revealing conditions for non-classical features and entanglement, paving the way for quantum information applications using high harmonics.
Contribution
It provides a closed-form theory of QSHHG in atoms and solids, identifying conditions for non-classical features and multi-mode entanglement in harmonic sidebands.
Findings
QSHHG results in multi-mode entanglement.
Projective measurement can generate non-classical states.
Conditions for realizing non-classical features are identified.
Abstract
In quantum sideband high harmonic generation (QSHHG), high harmonic generation is perturbed by a bright quantum field resulting in harmonic sidebands, with the intent to transfer non-classical properties from the quantum perturbation to the harmonic sidebands. So far, non-classical features have not been found in QSHHG yet. The closed form theory of QSHHG in atoms and solids developed here answers the question under which conditions non-classical features can be realized. QSHHG results in a multi-mode entanglement between harmonic sideband modes and perturbative quantum mode. A projective measurement on either creates a variety of non-classical states commonly used in quantum information science. This opens a pathway towards quantum engineering high harmonic generation as a short wavelength source for quantum information science.
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Taxonomy
TopicsLaser-Matter Interactions and Applications · Spectroscopy and Quantum Chemical Studies · Strong Light-Matter Interactions
