Universal temperature-dependent power law excitation gaps in frustrated quantum spin systems harboring order-by-disorder

TL;DR

This paper investigates how fluctuation-induced pseudo-Goldstone gaps in frustrated quantum spin systems depend on temperature, providing a universal power-law description that aids in detecting order-by-disorder phenomena in experiments.

Contribution

It introduces a formalism to compute the pseudo-Goldstone gap using linear spin-wave theory and reveals a universal power-law temperature dependence in frustrated quantum magnets.

Findings

Pseudo-Goldstone gap scales as T^{d+1} or T^{d/2+1} depending on dispersion.

Developed a simplified method using linear spin-wave theory.

Applied results to Er₂Ti₂O₇, supporting order-by-disorder detection.

Abstract

When magnetic moments are subject to competing or frustrated interactions, continuous degeneracies that are not protected by any symmetry of the parent Hamiltonian can emerge at the classical (mean-field) level. Such "accidental" degeneracies are often lifted by both thermal and quantum fluctuations via a mechanism known as order-by-disorder (ObD). The leading proposal to detect and characterize ObD in real materials, in a way that quantitatively distinguishes it from standard energetic selection, is to measure a small fluctuation-induced pseudo-Goldstone gap in the excitation spectrum. While the properties of this gap are known to leading order in the spin wave interactions, in both the zero-temperature and classical limits, the pseudo-Goldstone (PG) gap in quantum magnets at finite temperature has yet to be characterized. Using non-linear spin wave theory, we compute the PG gap to leading order in a $1/S$ expansion at low temperature for a variety of frustrated quantum spin systems. We also develop a formalism to calculate the PG gap in a way that solely uses linear spin-wave theory, circumventing the need to carry out tedious quantum many-body calculations. We argue that, at leading order, the PG gap acquires a distinct power-law temperature dependence, proportional to either $T^{d+1}$ or $T^{d/2+1}$ depending on the gapless dispersion of the PG mode predicted at the mean-field level. Finally, we examine the implications of these results for the pyrochlore oxide compound Er$_2$Ti$_2$O$_7$, for which there is compelling evidence of ObD giving rise to the experimentally observed long-range order.