Unraveling cavity-like modes of two-dimensional broad band hyperbolic metamaterial and their coupling to quantum emitters

TL;DR

This paper investigates cavity-like modes in two-dimensional hyperbolic metamaterials, demonstrating their properties, coupling to quantum emitters, and potential for enhancing light-matter interactions through experimental and theoretical analysis.

Contribution

It reveals the existence and characteristics of cavity-like modes in 2D HMMs and demonstrates their coupling to quantum emitters, advancing understanding beyond effective medium approximations.

Findings

Cavity-like modes persist despite Ohmic losses.

Experimental coupling to quantum emitters shows significant Purcell enhancement.

Mode volumes are confirmed by FDTD calculations.

Abstract

Hyperbolic metamaterials (HMM) are artificially engineered materials that exhibit hyperbolic dispersion of light propagating through them. These have been extensively studied for tailoring light propagation. Most studies use an effective medium approach that is extremely useful, though it misses out on properties that can arise from the microscopic details of the HMM. In particular, the HMM can have cavity-like modes, and it is important to understand such modes and their relevance in light propagation and coupling of HMM to quantum emitters. In this work, we bring out the cavity-like modes of the silver nanowire-alumina two-dimensional HMM, which remain on top of the broad response of the HMM. These modes define the characteristic reflection spectra. The observed resonances and their widths are in good agreement with our simulations. These well-defined modes occur even though the metallic part of the HMM has Ohmic losses. Then, we present experimental results on the coupling of quantum emitters to the cavity-like modes of the HMM. We present results for both steady-state and time-resolved photoluminescence. Using these, we extract the corresponding Purcell factors for radiative rate enhancement. Theoretical analyses of the experimental data allow the determination of the cavity coupling parameters and mode volumes. These experimental results are confirmed by the FDTD calculations for the HMM mode volume. This work elucidates the pathway to precise engineering for future applications of HMM modes in strong light-matter interactions.