U(1) Dirac quantum spin liquid candidate in triangular-lattice antiferromagnet CeMgAl$_{11}$O$_{19}$

TL;DR

This study provides experimental evidence for a U(1) Dirac quantum spin liquid state in the triangular-lattice antiferromagnet CeMgAl$_{11}$O$_{19}$, characterized by persistent spin fluctuations and gapless excitations.

Contribution

First detailed experimental investigation suggesting CeMgAl$_{11}$O$_{19}$ hosts a U(1) Dirac quantum spin liquid with persistent spin dynamics and gapless excitations.

Findings

No long-range magnetic order down to 50 mK

Persistent spin fluctuations at 1.0 MHz at 50 mK

Gapless excitations with power-law specific heat dependence

Abstract

Quantum spin liquid represents an intriguing state where electron spins are highly entangled yet spin fluctuation persists even at 0 K. Recently, the hexaaluminates \textit{R}MgAl$_{11}$O$_{19}$ (\textit{R} = rare earth) have been proposed to be a platform for realizing the quantum spin liquid state with dominant Ising anisotropic correlations. Here, we report detailed low-temperature magnetic susceptibility, muon spin relaxation, and thermodynamic studies on the CeMgAl$_{11}$O$_{19}$ single crystal. Ising anisotropy is revealed by magnetic susceptibility measurements. Muon spin relaxation and ac susceptibility measurements rule out any long-range magnetic ordering or spin freezing down to 50 mK despite the onset of spin correlations below $\sim$0.8 K. Instead, the spins keep fluctuating at a rate of 1.0(2) MHz at 50 mK. Specific heat results indicate a gapless excitation with a power-law dependence on temperature, $C_m(T) \propto T^{\alpha}$. The quasi-quadratic temperature dependence with $\alpha$ = 2.28(4) in zero field and linear temperature dependence in 0.25 T support the possible realization of the U(1) Dirac quantum spin liquid state.