PulseBat: A field-accessible dataset for second-life battery diagnostics from realistic histories using multidimensional rapid pulse test

TL;DR

PulseBat introduces a comprehensive dataset of second-life lithium-ion batteries tested under various pulse conditions, enabling improved diagnostics and safety assessments for battery reuse in energy-deprived regions.

Contribution

This work provides a large, diverse dataset of second-life batteries with detailed pulse test responses, facilitating advanced diagnostics and safety evaluation methods.

Findings

Recorded voltage and temperature responses under multiple pulse conditions.

Dataset covers various cathode types, usage histories, and physical formats.

Enables improved state-of-charge and state-of-health estimation methods.

Abstract

As electric vehicles (EVs) approach the end of their operational life, their batteries retain significant economic value and present promising opportunities for second-life use and material recycling. This is particularly compelling for Global South and other underdeveloped regions, where reliable energy storage is vital to addressing critical challenges posed by weak and even nonexistent power grid and energy infrastructures. However, despite this potential, widespread adoption has been hindered by critical uncertainties surrounding the technical performance, safety, and recertification of second-life batteries. In cases where they have been redeployed, mismatches between estimated and actual performance often render batteries technically unsuitable or hazardous, turning them into liabilities for communities they were intended to benefit. This considerable misalignment exacerbates energy access disparities and undermines the broader vision of energy justice, highlighting an urgent need for robust and scalable solutions to unlock the potential. In the PulseBat Dataset, the authors tested 464 retired lithium-ion batteries, covering 3 cathode material types, 6 historical usages, 3 physical formats, and 6 capacity designs. The pulse test experiments were performed repeatedly for each second-life battery with 10 pulse width, 10 pulse magnitude, multiple state-of-charge, and state-of-health conditions, e.g., from 0.37 to 1.03. The PulseBat Dataset recorded these test conditions and the voltage response as well as the temperature signals that were subject to the injected pulse current, which could be used as a valuable data resource for critical diagnostics tasks such as state-of-charge estimation, state-of-health estimation, cathode material type identification, open-circuit voltage reconstruction, thermal management, and beyond.