Combined Light Excitation and Scanning Gate Microscopy on Heterostructure Nanowire Photovoltaic Devices

TL;DR

This study combines light excitation with scanning gate microscopy on nanowire devices, enabling detailed analysis of optoelectronic behavior and defect states under realistic conditions.

Contribution

It introduces a novel setup integrating photoexcitation with high-resolution scanning gate microscopy for nanoscale optoelectronic device analysis.

Findings

Observation of negative and positive photoconductance effects.

Ability to distinguish effects of composition and surface states.

Model predictions align with experimental results.

Abstract

Nanoscale optoelectronic components achieve functionality via spatial variation in electronic structure induced by composition, defects, and dopants. To dynamically change the local band alignment and influence defect states, a scanning gate electrode is highly useful. However, this technique is rarely combined with photoexcitation by a controlled external light source. We explore a setup that combines several types of light excitation with high resolution scanning gate and atomic force microscopy (SGM/AFM). We apply the technique to InAs nanowires with an atomic scale defined InP segment, that have attracted considerable attention for studies of hot carrier devices. Using AFM we image the topography of the nanowire device. SGM measurements without light excitation show how current profiles can be influenced by local gating near the InP segment. Modelling of the tip and nanowire can well predict the results based on the axial band structure variation and an asymmetric tip. SGM studies including light excitation are then performed using both a white light LED and laser diodes at 515 and 780nm. Both negative and positive photoconductance can be observed and the combined effect of light excitation and local gating is observed. SGM can then be used to discriminate between effects related to the wire axial compositional structure and surface states. The setup explored in the current work has significant advantages to study optoelectronics at realistic conditions and with rapid turnover.