Circular Dichroism in Resonant Inelastic X-ray Scattering: Probing Altermagnetic Domains in MnTe
D. Takegami, T. Aoyama, T. Okauchi, T. Yamaguchi, S. Tippireddy, S. Agrestini, M. Garc\'ia-Fern\'andez, T. Mizokawa, K. Ohgushi, Ke-Jin Zhou, J. Chaloupka, J. Kune\v{s}, A. Hariki, H. Suzuki

TL;DR
This paper demonstrates that resonant inelastic X-ray scattering circular dichroism (RIXS-CD) can effectively identify and distinguish altermagnetic domains in MnTe by detecting mirror-symmetry breaking and domain occupation through azimuthal dependence.
Contribution
It introduces RIXS-CD as a novel, domain-sensitive technique for probing altermagnetic order and elementary excitations in quantum materials.
Findings
RIXS-CD reveals dominant occupation of a single altermagnetic domain.
Azimuthal dependence indicates mirror-symmetry breaking.
RIXS-CD can differentiate magnetic domains related by crystallographic symmetries.
Abstract
X-ray magnetic circular dichroism provides a means to identify ferromagnetic, chiral, and altermagnetic orders via their time-reversal-symmetry () breaking. However, differentiating magnetic domains related by crystallographic symmetries remains a technical challenge. Here we reveal a circular dichroism (CD) in the resonant inelastic x-ray scattering (RIXS) spectra from the altermagnetic MnTe. The azimuthal dependence of the RIXS-CD intensity of the magnon excitations indicates a dominant occupation of a single altermagnetic domain. The RIXS-CD in our scattering geometry is ascribed to the mirror-symmetry breaking associated with the -broken altermagnetic order. Our results establish RIXS-CD as a domain-sensitive probe of elementary excitations in quantum materials.
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Taxonomy
TopicsX-ray Diffraction in Crystallography · Crystallography and Radiation Phenomena · Magnetic properties of thin films
