Fragile Unconventional Magnetism in RuO$_2$ by Proximity to Landau-Pomeranchuk Instability

TL;DR

This paper reveals that RuO$_2$ exhibits altermagnetism as a form of unconventional magnetism near a Landau-Pomeranchuk instability, with its magnetic properties tunable via external parameters, offering insights into quantum phase transitions.

Contribution

The study demonstrates, through first-principles calculations, that RuO$_2$'s altermagnetism is linked to its proximity to a quantum phase transition and explores how tuning parameters affect its magnetic state.

Findings

RuO$_2$'s altermagnetism is near a quantum phase transition.

Tuning parameters like Hubbard U, doping, and strain modulate magnetic interactions.

Reconciliation of conflicting experimental and theoretical reports on RuO$_2$'s magnetism.

Abstract

Altermagnetism has attracted considerable attention for its remarkable combination of spin-polarized band structures and zero net magnetization, making it a promising candidate for spintronics applications. We demonstrate that this magnetic phase represents a case of ``unconventional magnetism," first proposed nearly two decades ago by one of the present authors as part of a broader framework for understanding Landau-Pomeranchuk instabilities in the spin channel, driven by many-body interactions. By systematically analyzing the altermagnetism in RuO$_2$ with first-principles calculations, we reconcile conflicting experimental and theoretical reports by attributing it to RuO$_2$'s proximity to a quantum phase transition. We emphasize the critical role of tuning parameters, such as the Hubbard $U$, hole doping, and epitaxial strain, in modulating quasiparticle interactions near the Fermi surface. This work provides fresh insights into the origin and tunability of altermagnetism in RuO$_2$, highlighting its potential as a platform for investigating quantum phase transitions and the broader realm of unconventional magnetism.