Lifetime measurement of the 5s5p 1P1 state in strontium

TL;DR

This paper reports a precise measurement of the lifetime of the $5s5p~^1P_1$ state in strontium using time-correlated single-photon counting with femtosecond laser excitation, achieving high accuracy by thoroughly analyzing systematic effects.

Contribution

It provides the first direct lifetime measurement of the $^1P_1$ state in strontium with improved accuracy and detailed systematic error analysis.

Findings

Measured lifetime of $^1P_1$ state: 5.216 ns

Achieved high signal-to-noise ratio with femtosecond pulsed laser

Systematic effects thoroughly analyzed and minimized

Abstract

We present a direct lifetime measurement of the $5s5p~^1P_1$ state of strontium using time-correlated single-photon counting of laser induced fluorescence in a hot atomic beam. To achieve fast switch-off times and a high signal-to-noise ratio, we excite the strontium atoms with a femtosecond pulsed laser at $\approx$461 nm and collect the fluorescence onto a hybrid single-photon detector. Analysis of the measured exponential decay gives a lifetime of the $^1P_1$ state of $\tau = (5.216 \pm 0.006_{stat} \pm 0.013_{sys})$ ns, where all the systematic effects have been thoroughly considered.