X-Ray-Driven Photon Bunching

TL;DR

This paper demonstrates how photon bunching analysis, rooted in HBT interferometry, can be used to characterize scintillation properties of various materials, including nanoscale scintillators, revealing new insights into their light emission mechanisms.

Contribution

It introduces a novel method linking photon bunching to scintillation characterization, applicable to nano- and micro-scale materials, and benchmarks this approach across diverse scintillators.

Findings

Intrinsic photon bunching observed in scintillation processes.

Quantitative extraction of scintillation lifetime and light yield.

Strong photon bunching (g^{(2)}(0)>50) in nanocrystals.

Abstract

Hanbury Brown and Twiss (HBT) interferometry is a milestone experiment that transformed our understanding of the nature of light. The concept was demonstrated in 1956 to measure the radii of stars through photon coincidence detection. This form of coincidence detection later became a cornerstone of modern quantum optics. Here we connect HBT interferometry to the physics of scintillation, the process of spontaneous light emission upon excitation by high-energy particles, such as x-rays. Our work reveals intrinsic photon bunching in the scintillation process, which we utilize to elucidate its underlying light emission mechanisms. Specifically, g^((2) ) ({\tau}) enables the quantitative extraction of scintillation lifetime and light yield, showing their dependence on temperature and X-ray flux as well. This approach provides a characterization method that we benchmark on a wide gamut of scintillators, including rare-earth-doped garnets and perovskite nanocrystals. Our method is particularly important for nano- and micro-scale scintillators, whose properties are challenging to quantify by conventional means: We extract the scintillation properties in perovskite nanocrystals of only a few hundreds of nanometers, observing strong photon bunching (g^((2) ) (0)>50). Our research paves the way for broader use of photon-coincidence measurement and methods from quantum optics in studying materials with complex optical properties in extremes regions of the electromagnetic spectrum.