Altermagnetism and Strain Induced Altermagnetic Transition in Cairo Pentagonal Monolayer

TL;DR

This paper introduces a new two-dimensional altermagnetic system based on Cairo pentagonal monolayers, demonstrating strain-induced transitions and potential for spintronic applications through theoretical models and ab initio calculations.

Contribution

It presents a novel Cairo pentagonal monolayer system exhibiting g-wave to d-wave altermagnetic transition induced by strain, with a realistic tight-binding model and topological properties analysis.

Findings

Strain induces a transition from g-wave to d-wave altermagnetism.

Non-trivial band topology can be realized by symmetry breaking.

Candidate materials like FeS₂ and Nb₂FeB₂ exhibit the proposed properties.

Abstract

Altermagnetism, a recently discovered class of magnetic order characterized by vanishing net magnetization and spin-splitting band structures, has garnered significant research attention. In this work, we introduce a novel two-dimensional system that exhibits $g$-wave altermagnetism and undergoes a strain-induced transition from $g$-wave to $d$-wave altermagnetism. This system can be realized in an unconventional monolayer Cairo pentagonal lattice, for which we present a realistic tight-binding model that incorporates both magnetic and non-magnetic sites. Furthermore, we demonstrate that non-trivial band topology can emerge in this system by breaking the symmetry that protects the spin-polarized nodal points. Finally, \emph{ab initio} calculations on several candidate materials, such as FeS$_2$ and Nb$_2$FeB$_2$, which exhibit symmetry consistent with the proposed tight-binding Hamiltonian, are also presented. These findings open new avenues for exploring spintronic devices based on altermagnetic systems.