Magnetic field tuned superconducting and normal phase magnetism in CeCo$_{0.5}$Rh$_{0.5}$In$_{5}$

TL;DR

This study investigates how magnetic fields influence the magnetic and superconducting phases in CeCo$_{0.5}$Rh$_{0.5}$In$_{5}$, revealing field-dependent static magnetism and anisotropic behavior in the material.

Contribution

It provides new insights into the field-tuned magnetic phases and anisotropic responses in CeCo$_{0.5}$Rh$_{0.5}$In$_{5}$, especially regarding the emergence of incommensurate magnetism.

Findings

Magnetic field along the c-axis does not change static magnetism.

In-plane magnetic fields increase the Néel temperature and alter magnetic responses.

Intermediate fields induce commensurate block magnetism with a specific propagation vector.

Abstract

By tuning superconductivity with an applied magnetic field, we use neutrons to compare the magnetic ordered phases in superconducting and normal states of CeCo$_{0.5}$Rh$_{0.5}$In$_{5}$. At zero field, CeCo$_{0.5}$Rh$_{0.5}$In$_{5}$ displays both superconductivity ($T_{c}$=1.3 K) and spatially long-ranged commensurate $\uparrow\downarrow\uparrow\downarrow$ antiferromagnetism ($T_{N}$=2.5 K, $\vec{Q}_{0}=({1\over 2}, {1\over 2}, {1\over 2})$). Neutron spectroscopy fails to measure propagating magnetic excitations with only temporally overdamped fluctuations observable. On applying a magnetic field we find anisotropic behavior in the static magnetism. When the field is along the crystallographic $c$-axis, no change in the static magnetic response is observable. However when the field is oriented within the $a-b$ plane, an increase in $T_{N}$ and change in the critical response are measured. At low temperatures in the superconducting phase, the elastic magnetic intensity increases linearly ($\propto |H|$) with small $a-b$ oriented fields. However, this trend is interrupted at intermediate fields where commensurate block $\uparrow\uparrow\downarrow\downarrow$ magnetism with propagation vector $\vec{Q}=({1\over 2}, {1\over 2}, {1\over 4})$ forms. For large applied fields in the [1 $\overline{1}$ 0] direction which completely suppresses superconductivity, weakly incommensurate magnetic order along $L$ is observed to replace the commensurate response present in the superconducting and vortex phases. We suggest field-induced incommensurate static magnetism, present in the normal state of superconducting and antiferromagnetic CeCo$_{0.5}$Rh$_{0.5}$In$_{5}$ for $a-b$ plane oriented magnetic fields. We speculate that these field dependent properties are tied to the field induced anisotropy associated with the local Ce$^{3+}$ crystal field environment of the tetragonal `115' structure.