Dense Suspensions in Rotary Shear

TL;DR

This paper introduces a novel Rotary Shear (RS) protocol for dense suspensions, revealing unique irreversible dynamics and microstructure behavior distinct from classical oscillatory shear, with implications for understanding suspension rheology.

Contribution

The study presents the Rotary Shear protocol and demonstrates its effects on suspension dynamics and microstructure, highlighting differences from traditional oscillatory shear methods.

Findings

RS protocol prevents self-adsorbing states and reversible-irreversible transition.

Suspensions under RS exhibit always diffusive, irreversible dynamics.

Microstructure analysis shows persistent anisotropy without a reversible transition.

Abstract

We introduce a novel unsteady shear protocol, which we name Rotary Shear (RS), where the flow and vorticity directions are continuously rotated around the velocity gradient direction by imposing two out-of-phase oscillatory shear (OS) in orthogonal directions. We perform numerical simulations of dense suspensions of rigid non-Brownian spherical particles at volume fractions ($\phi$) between 0.40 and 0.55 subject to this new RS protocol and compare to the classical OS protocol. We find that the suspension viscosity displays a similar non-monotonic response as the strain amplitude ($\gamma_0$) is increased: a minimum viscosity is found at an intermediate, volume-fraction dependent strain amplitude. However, the suspension dynamics is different in the new protocol. Unlike the OS protocol, suspensions under RS do not show self-adsorbing states at any $\gamma_0$ and do not undergo the reversible-irreversible transition: the stroboscropic particle dynamics are always diffusive, which we attribute to the fact that the RS protocol is irreversible. To validate this hypothesis, we introduce a reversible-RS (RRS) protocol, a combination of RS and OS, where we rotate the shear direction (as in RS) until it is instantaneously reversed (as in OS), and find the resulting rheology and dynamics to be closer to OS. Detailed microstructure analysis shows that both the OS and RRS protocols result in a contact-free, isotropic to an in-contact, anisotropic microstructure at the dynamically reversible-to-irreversible transition. The RS protocol does not render such a transition, and the dynamics remain diffusive with an in-contact, anisotropic microstructure for all strain amplitudes.