Multiscale stress dynamics in sheared liquid foams revealed by tomo-rheoscopy

TL;DR

This study combines shear rheometry and X-ray micro-tomography to investigate multiscale stress dynamics in sheared liquid foams, revealing universal scaling laws and non-local stress redistribution mechanisms at the bubble level.

Contribution

It introduces a novel experimental approach to measure local stresses and topology in 3D liquid foams, uncovering the link between microstructural rearrangements and macroscopic elastoplastic behavior.

Findings

Universal scaling of local stress build-up and relaxation.

Stress redistribution exhibits quadrupolar patterns.

Microstructural rearrangements drive macroscopic rheological response.

Abstract

Rheology aims at quantifying the response of materials to mechanical forcing. However, standard rheometers provide only global macroscopic quantities, such as viscoelastic moduli. They fail to capture the heterogeneous flow of soft amorphous materials at the mesoscopic scale, arising from the rearrangements of the microstructural elements, that must be accounted for to build predictive models. To address this experimental challenge, we have combined shear rheometry and time-resolved X-ray micro-tomography on 3D liquid foams used as model glassy materials, yielding a unique access to the stresses and contact network topology at the bubble scale. We reveal a universal scaling behavior of the local stress build-up and relaxation associated with topological modifications. Moreover, these plastic events redistribute stress non-locally, as if the foam were an elastic medium subjected to a quadrupolar deformation. Our findings clarify how the macroscopic elastoplastic behavior of amorphous materials emerges from the spatiotemporal stress variations induced by microstructural rearrangements.