Magnetization process of a quasi-two-dimensional quantum magnet: Two-step symmetry restoration and dimensional reduction

TL;DR

This study investigates the magnetization process in a quasi-2D quantum magnet, revealing a two-step symmetry restoration and dimensional reduction through experimental and numerical analysis of phase transitions and magnetization plateaus.

Contribution

It provides new insights into the field-induced phase transitions and symmetry restoration in a quasi-2D quantum magnet using combined experimental and quantum Monte Carlo simulations.

Findings

Identification of a field-induced transition at 16.3 T with a magnetization plateau.

Demonstration that full polarization occurs at approximately 95 T, indicating a 1D quantum phase transition.

Evidence that the observed phase transition results from partial symmetry restoration and dimensional reduction.

Abstract

We report on a comprehensive thermodynamic study of a quasi-two-dimensional (quasi-2D) quantum magnet Cu$_2$(OH)$_3$Br which in the 2D layer can be viewed as strongly coupled alternating antiferromagnetic and ferromagnetic chains. In an applied magnetic field transverse to the ordered spins below $T_N=9.3$ K, a field-induced phase transition from the 3D ordered to a disordered phase occurs at $B_c=16.3$ T for the lowest temperature, which is featured by an onset of a one-half plateau-like magnetization. By performing quantum Monte Carlo simulations of the relevant 2D model, we find that the plateau-like magnetization corresponds to a partial symmetry restoration and the full polarization in the ferromagnetic chains. Our numerical simulations also show that the magnetization saturation occurs with full symmetry restoration at a much higher field of $B_s \simeq 95$ T, corresponding to a 1D quantum phase transition in the antiferromagnetic chains. We argue that the experimentally observed field-induced phase transition at $B_c$ follows from the partial symmetry restoration and the concomitant dimensional reduction.