Cs-O$_2$-Li as enhanced NEA surface layer with increased lifetime for GaAs photocathodes

TL;DR

This research introduces a Cs-O$_2$-Li surface layer for GaAs photocathodes, significantly increasing their operational lifetime and charge extraction without compromising efficiency, thus advancing spin-polarized electron sources.

Contribution

The paper demonstrates that incorporating Li during activation forms an enhanced NEA layer, markedly improving photocathode durability and performance over previous methods.

Findings

Lifetime increased by up to 19 times

Charge extraction improved by up to 16.5 times

No significant reduction in quantum efficiency

Abstract

GaAs-based photocathodes are the only viable source capable of providing spin-polarized electrons for accelerator applications. This type of photocathode requires a thin surface layer, in order to achieve negative electron affinity (NEA) for efficient photo-emission. However, this layer is vulnerable to environmental and operational effects, leading to a decay of the quantum efficiency $\eta$ characterized by a decay constant or lifetime $\tau$. In order to increase $\tau$, additional agents can be introduced during the activation procedure to improve the chemical robustness of the surface layer. This paper presents the results of recent research on Li as enhancement agent for photocathode activation using Cs and O$_2$, forming Cs-O$_2$-Li as enhanced NEA layer. Measurements yielded an increase in lifetime by a factor of up to 19 $\pm$ 2 and an increase in extracted charge by a factor of up to 16.5 $\pm$ 2.4, without significant reduction of $\eta$. This performance is equal to or better than that reported for other enhanced NEA layers so far.