A tutorial on THz pulse analysis: accurate retrieval of pulse arrival times, spectral energy density and absolute spectral phase

TL;DR

This paper reviews Fourier analysis techniques for THz pulse measurement, introduces a phenomenological model for pulse reproduction, and presents methods for accurate spectral phase and timing retrieval in time-domain spectroscopy.

Contribution

It provides a comprehensive tutorial on THz pulse analysis, emphasizing best practices in Fourier analysis and introducing a model for diverse pulse types.

Findings

Validated a phenomenological model for THz pulses

Demonstrated accurate spectral phase retrieval methods

Compared spectral energy densities across sources

Abstract

Electro-optic sampling allows the electric field of THz, mid-infrared and visible light pulses to be measured directly as a function of time, with data analysis often performed in the frequency domain after fast Fourier transform. Here we review aspects of Fourier theory relevant to the frequency-domain analysis of light pulses recorded in the time-domain. We describe a ``best practise'' approach to using the discrete Fourier transform that ensures consistency with analytical results from the continuous Fourier transform. We summarise a phenomenological time-domain model of THz pulses, based on carrier and envelope waves, and show that it can reproduce a wide variety of experimental single- to multi-cycle THz pulses, with exemplary data from lab-based sources (photoconductive antennae, optical rectification, spintronic emitters) and a THz free electron laser. A quantitative comparison of the spectral energy density of these distinct sources is enabled by the amplitude-accuate discrete Fourier transform. We describe a method that ensures the accurate calculation of the absolute spectral phase (valid for arbitrary sampling windows in the time-domain) and summarise how the carrier-envelope phase, pulse arrival time and chirp can be obtained from the phase. Our aim with this overview of THz pulse analysis is to highlight algorithms and concepts that are useful to newcomers to time-domain spectroscopy and experts, alike.