Connection between f-electron correlations and magnetic excitations in UTe2
Thomas Halloran, Peter Czajka, Gicela Saucedo Salas, Corey Frank,, Chang-Jong Kang, J.A. Rodriguez-Rivera, Jakob Lass, Daniel G. Mazzone, Marc, Janoschek, Gabi Kotliar, Nicholas P. Butch

TL;DR
This study uses inelastic neutron scattering to explore the anisotropic magnetic excitations in UTe2, revealing their origin from f-electron hybridization and their behavior under magnetic fields, contributing to understanding its superconducting properties.
Contribution
It provides detailed insights into the anisotropic magnetic excitations and their relation to f-electron correlations in UTe2, a candidate spin-triplet superconductor.
Findings
Magnetic excitations originate from the Brillouin zone boundary at Y and T points.
Magnetism remains field-independent up to 11 T along the c-axis.
Excitations are consistent with U3+/U4+ f-electron spins with a fluctuating moment of 2.3 μB.
Abstract
The detailed anisotropy of the low-temperature, low-energy magnetic excitations of the candidate spin-triplet superconductor UTe is revealed using inelastic neutron scattering. The magnetic excitations emerge from the Brillouin zone boundary at the high symmetry and points and disperse along the crystallographic -axis. In applied magnetic fields to at least ~T along the axis, the magnetism is found to be field-independent in the plane. The scattering intensity is consistent with that expected from U/U -electron spins with preferential orientation along the crystallographic -axis, and a fluctuating magnetic moment of 2.3(7) . These characteristics indicate that the excitations are due to intraband spin excitons arising from -electron hybridization.
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Taxonomy
TopicsRare-earth and actinide compounds · Radioactive element chemistry and processing · Catalysis and Oxidation Reactions
