Correlation of Magnetic State Configurations in Nanotubes with FMR spectrum

TL;DR

This paper uses RFMR spectroscopy and micromagnetic simulations to characterize magnetic configurations in nanotubes, revealing distinct spin states and their evolution under different magnetic field orientations.

Contribution

It introduces a combined experimental and simulation approach to identify and analyze various magnetic states in nanotubes using RFMR and FMR spectra.

Findings

Distinct spin configurations identified, including vortex, onion, and curling states.

RFMR spectra correspond to specific magnetic configurations and their evolution.

Magnetic states depend on field orientation and bias, with corroboration from FORC measurements.

Abstract

Magnetic nanotubes have garnered immense attention for their potential in high-density magnetic memory, owing to their stable flux closure configuration and fast, reproducible reversal processes. However, characterizing their magnetic configuration through straightforward methodologies remains a challenge in both scope and detail. Here, we elucidate the magnetic state details using Remanence Field Ferromagnetic Resonance Spectroscopy (RFMR) for arrays of electrodeposited nanotubes. Micromagnetic simulations revealed distinct spin configurations while coming from saturation, including the edge vortex, onion, uniform and curling states, with chirality variations depending on the preparation field direction. Dynamic measurements, coupled with RFMR spectra analysis, unveiled multiple FMR modes corresponding to these spin configurations. The evolution of spin configurations under bias fields were studied, indicating nucleation within the curling state. Observations revealed opposite RFMR spectra, denoting opposite magnetic spin configurations after removing the positive and negative saturating fields when the magnetic field was applied along {theta_H=0} and perpendicular {theta_H= 90} to the nanotube axis. We observed a mixture of the non-uniform curling states with the end vortex state (onion-like curling state) at the end of the nanotubes for the theta_H=0(90) and uniform magnetization states in the middle of the nanotubes for the theta_H=0 configuration. Building on RFMR information, frequency-swept FMR absorption spectra obtained at different bias fields allowed the characterization of magnetization states. This picture was supported by micromagnetic simulations. These findings were further substantiated with First Order Reversal Curve measurements (FORC).