Tunneling maps, non-monotonic resistivity, and non Drude optics in EuB$_6$

TL;DR

This paper models EuB$_6$ using a Heisenberg-Kondo lattice to explain its non-monotonic resistivity, spatial textures, and non-Drude optical response, revealing temperature-dependent electronic and magnetic textures.

Contribution

It provides a comprehensive theoretical explanation for EuB$_6$'s unusual properties using exact diagonalisation-based Langevin dynamics, linking textures to transport and optical phenomena.

Findings

Observation of electronic and magnetic textures matching experimental scales

Confirmation of non-monotonic resistivity near $T_c$

Prediction of non-Drude optical conductivity in the polaronic phase

Abstract

For several decades the low carrier density local moment magnet EuB$_6$ has been considered a candidate material for ferromagnetic polarons. There is however no consistent explanation for the host of intriguing observations that have accrued over the years, including a prominently non-monotonic resistivity near $T_c$, and observation of spatial textures, with a characteristic spatial and energy scale, via scanning tunneling spectroscopy. We resolve all these features using a Heisenberg-Kondo lattice model for EuB$_6$, solved using exact diagonalisation based Langevin dynamics. Over a temperature window $\sim 0.7T_c - 1.5T_c$ we observe electronic and magnetic textures with the correct spatial and energy scale, and confirm an associated non-monotonic resistivity. We predict a distinctly `non Drude' optical conductivity in the polaronic phase, and propose a field-temperature phase diagram testable through spin resolved tunneling spectroscopy. We argue that the anomalous properties of EuB$_6$, and magnetic polaron materials in general, occur due to a non monotonic change in spatial character of `near Fermi level' eigenstates with temperature, and the appearance of a weak pseudogap near $T_c$.