The Origin of Sound Damping in Amorphous Solids: Defects and Beyond

TL;DR

This paper investigates the microscopic origins of sound damping in amorphous solids, revealing that both defects and non-affine forces contribute to attenuation, challenging traditional defect-centric models.

Contribution

It introduces a particle-level analysis of sound damping, identifying defect regions and non-defect contributions, and proposes a new paradigm for understanding sound attenuation in glasses.

Findings

Sound damping scales linearly with defect fraction in glasses.

Ultra-stable glasses exhibit damping due to non-affine forces without defects.

Defects are not solely responsible for Rayleigh scattering in glasses.

Abstract

Comprehending sound damping is integral to understanding the anomalous low temperature properties of glasses. After decades of theoretical and experimental studies, Rayleigh scattering scaling of the sound attenuation coefficient with frequency, $\Gamma \sim \omega^{d+1}$, became generally accepted when quantum and finite temperature effects can be neglected. Rayleigh scaling invokes a picture of scattering from defects. However, it is unclear how to define glass defects, or even if defects are necessary for Rayleigh scaling. Here we determine a particle level contribution to sound damping in the Rayleigh scaling regime. We find that there are areas in the glass that contribute more to sound damping than other areas over a range of frequencies, which allows us to define defects. We show that over a range of glass stability, sound damping scales linearly with the fraction of particles in the defects. However, sound is still attenuated in ultra-stable glasses where no defects are identified. We show that sound damping in these glasses is due to nearly uniformly distributed non-affine, microscopic forces that arise after macroscopic deformations of non-centrosymetric structures. To fully understand sound attenuation in glasses one has to consider contributions from defects and a defect-free background, which represents a new paradigm of sound damping in glasses.