Self-induced spin pumping and inverse spin Hall effect in single FePt thin films

TL;DR

This paper demonstrates self-induced spin pumping and inverse spin Hall effect in single FePt thin films, revealing their efficiency and mechanisms, and compares them to platinum, advancing spintronics device development.

Contribution

It introduces the observation of self-induced spin-charge conversion in single FePt films and quantifies their spin Hall parameters, providing new insights into spin-to-charge conversion mechanisms.

Findings

Self-induced spin pumping voltage observed in FePt films.

Quantified spin Hall angle and spin diffusion length for FePt.

Independent extraction of FePt and Pt contributions in bilayer systems.

Abstract

In this study, we investigate the spin-charge current conversion characteristics of chemically disordered ferromagnetic single FePt thin films by spin-pumping ferromagnetic resonance experiments performed on both a resonance cavity and on patterned devices. We clearly observe a self-induced signal in a single FePt layer. The sign of a single FePt spin pumping voltage signal is consistent with a typical bilayer with a positive spin Hall angle layer such as that of Pt on top of a ferromagnet (FM), substrate//FM/Pt. Structural analysis shows a strong composition gradient due to natural oxidation at both FePt interfaces, with the Si substrate and with the air. The FePt-thickness dependence of the self-induced charge current produced allowed us to obtain $\lambda _ \text{FePt}=(1.5\pm 0.1)$ nm and self-induced $\theta_ \text{self-FePt}=0.047 \pm 0.003$, with efficiency for reciprocal effects applications $\theta _ \text{self-FePt} \times \lambda _ \text{FePt} = 0.071$ nm which is comparable to that of Pt, $\theta _ \text{SH-Pt} \times \lambda _ \text{Pt} = 0.2$ nm. Moreover, by studying bilayer systems such as Si//FePt/Pt and Si//Pt//FePt we independently could extract the individual contributions of the external inverse spin Hall effect of Pt and the self-induced inverse spin Hall effect of FePt. Notably, this method gives consistent values of charge currents produced due to only self-induced inverse spin Hall effect in FePt layers. These results advance our understanding of spin-to-charge interconversion mechanisms in composite thin films and pave the way for the development of next-generation spintronics devices based on self-torque.