Bridging Rayleigh-Jeans and Bose-Einstein condensation of a guided fluid of light with positive and negative temperatures

TL;DR

This paper unifies the thermodynamics of Rayleigh-Jeans and Bose-Einstein condensations of light in waveguides, introducing a frequency cut-off to derive generalized properties and exploring negative temperature regimes.

Contribution

It introduces a frequency cut-off to reconcile classical and quantum light condensation thermodynamics, extending the framework to include negative temperatures.

Findings

Derived generalized thermodynamic expressions for light condensation.

Reconciled differences between Rayleigh-Jeans and Bose-Einstein condensation behaviors.

Explored negative temperature regimes with non-critical specific heat behavior.

Abstract

We consider the free propagation geometry of a light beam (or fluid of light) in a multimode waveguide. As a result of the effective photon-photon interactions, the photon fluid thermalizes to an equilibrium state during its conservative propagation. In this configuration, Rayleigh-Jeans (RJ) thermalization and condensation of classical light waves have been recently observed experimentally in graded index multimode optical fibers characterized by a 2D parabolic trapping potential. As well-known, the properties of RJ condensation differ substantially from those of Bose-Einstein (BE) condensation: The condensate fraction decreases quadratically with the temperature for BE condensation, while it decreases linearly for RJ condensation. Furthermore, for quantum particles the heat capacity tends to zero at small temperatures, and it takes a constant value in the classical particle limit at high temperatures. This is in contrast with classical RJ waves, where the specific heat takes a constant value at small temperatures, and tends to vanish above the condensation transition in the normal (uncondensed) state. Here, we reconcile the thermodynamic properties of BE and RJ condensation: By introducing a frequency cut-off inherent to light propagation in a waveguide, we derive generalized expressions of the thermodynamic properties that include the RJ and BE limits as particular cases. We extend the approach to encompass negative temperatures. In contrast to positive temperatures, the specific heat does not display a singular behavior at negative temperatures, reflecting the non-critical nature of the transition to a macroscopic population of the highest energy level. Our work contributes to understanding the quantum-to-classical crossover in the equilibrium properties of light, within a versatile experimental platform based on nonlinear optical propagation in multimode waveguides.