Quantum Oscillations in kagome metals CsTi3Bi5 and RbTi3Bi5

TL;DR

This study investigates quantum oscillations in kagome metals CsTi3Bi5 and RbTi3Bi5, revealing new frequencies and comparing experimental results with theoretical calculations to understand their electronic structures.

Contribution

It reports the first observation of multiple unreported quantum oscillation frequencies in CsTi3Bi5 and compares these with density functional theory calculations, highlighting similarities and differences between the two compounds.

Findings

Multiple unreported frequencies above 2000 T in CsTi3Bi5

Good agreement between experimental data and DFT calculations for CsTi3Bi5

Different quantum oscillation spectra observed in RbTi3Bi5

Abstract

We report quantum oscillation measurements on the kagome compounds ATi$_3$Bi$_5$ (A=Rb, Cs) in magnetic fields up to 41.5 T and temperatures down to 350 mK. In addition to the frequencies observed in previous studies, we have observed multiple unreported frequencies above 2000 T in CsTi$_3$Bi$_5$ using a tunnel diode oscillator technique. We compare these results against density functional theory calculations and find good agreement with the calculations in the number of peaks observed, frequency, and the dimensionality of the Fermi surface. For RbTi$_3$Bi$_5$ we have obtained a different quantum oscillation spectrum, although calculated quantum oscillation frequencies for the Rb compound are remarkably similar to the Cs compound, calling for further studies.