A broadband pulse amplifier for Joule heating experiments in diamond anvil cells

TL;DR

This paper introduces a novel broadband pulse amplifier designed for Joule heating experiments in diamond anvil cells, enabling precise, high-temperature heating of tiny metal samples under megabar pressures.

Contribution

The paper presents the design and characterization of a new pulse amplifier capable of heating metal wires to thousands of kelvin at megabar pressures within diamond anvil cells, with adjustable pulse parameters.

Findings

Able to heat metal wires to thousands of kelvin

Provides accurate resistance measurements within 5%

Operates over a wide range of pulse durations and currents

Abstract

Decades of measurements of the thermophysical properties of hot metals show that pulsed Joule heating is an effective method to heat solid and liquid metals that are chemically reactive or difficult to contain. In order to extend such measurements to megabar pressures, pulsed heating methods must be integrated with diamond anvil cells. We report the design and characterization of a new pulse amplifier that can heat $\sim 5$ to $50$ $\mu$m-diameter metal wires to 1000s of kelvin at megabar pressures using diamond anvil cells. Pulse durations and peak currents can each be varied over 3 orders of magnitude, from 5 $\mu$s to 10 ms and 0.2 to 200 A. The pulse amplifier is integrated with a current probe. Two voltage probes attached to the body of a diamond anvil cell can be used to measure voltage in a four point probe geometry. The accuracy of four point probe resistance measurements for a dummy sample with 0.1 $\Omega$ resistance are typically better than $5 \%$ at all times from 2 $\mu$s to 10 ms after the beginning of the pulse.