Transport Study of Charge Carrier Scattering in Monolayer WSe$_2$
Andrew Y. Joe, Kateryna Pistunova, Kristen Kaasbjerg, Ke Wang, Bumho, Kim, Daniel A. Rhodes, Takashi Taniguchi, Kenji Watanabe, James Hone, Tony, Low, Luis A. Jauregui, and Philip Kim

TL;DR
This study investigates charge carrier scattering in high-quality monolayer WSe$_2$ transistors, revealing non-monotonic mobility behavior and demonstrating quantized conductance, which highlights the potential for advanced quantum optoelectronic applications.
Contribution
It provides the first detailed quantum transport analysis of defect-related scattering in monolayer WSe$_2$, linking energy-dependent scattering to mobility behavior and demonstrating device quality through quantized conductance.
Findings
Non-monotonic mobility as a function of hole density.
Energy-dependent scattering amplitude explains mobility behavior.
Observation of quantized conductance steps in quantum point contacts.
Abstract
Employing flux-grown single crystal WSe, we report charge carrier scattering behaviors measured in -BN encapsulated monolayer field effect transistors. We perform quantum transport measurements across various hole densities and temperatures and observe a non-monotonic change of transport mobility as a function of hole density in the degenerately doped sample. This unusual behavior can be explained by energy dependent scattering amplitude of strong defects calculated using the T-matrix approximation. Utilizing long mean-free path (500 nm), we demonstrate the high quality of our electronic devices by showing quantized conductance steps from an electrostatically-defined quantum point contact. Our results show the potential for creating ultra-high quality quantum optoelectronic devices based on atomically thin semiconductors.
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Taxonomy
Topics2D Materials and Applications · Molecular Junctions and Nanostructures · Semiconductor materials and interfaces
