Correlation of Blocking and N\'eel Temperatures in Ultra-thin Metallic Antiferromagnets

TL;DR

This study investigates the relationship between blocking and Ne9el temperatures in ultrathin metallic antiferromagnets using spin pumping and magnetometry, providing insights crucial for scalable antiferromagnetic spintronics.

Contribution

It introduces a method to correlate blocking and Ne9el temperatures in ultrathin antiferromagnetic layers through spin pumping and magnetometry measurements.

Findings

Temperature shifts in resonance peaks indicate the blocking temperature.

Blocking and Ne9el temperatures are correlated in ultrathin layers.

Thickness influences thermal stability of antiferromagnets.

Abstract

Nonvolatile spintronics-based devices that utilize electron spin both to store and transport information face a great challenge when scaled to nano dimensions due to loss of thermal stability and stray field induced disturbance in closely packed magnetic bits. The potential replacement of ferromagnetic materials with antiferromagnets may overcome some of these issues owing to the superior robustness of sublattice spin orientations to magnetic field disturbance as long as theyare kept well below the N\'eel temperature, which is hard to measure with conventional methods, especially in the ultrathin limit. In this work, we have employed spin pumping from a soft ferromagnetic NiFe layer into widely used ultrathin metallic antiferromagnet Ir20Mn80, FeMn, PtMn, PdMn or NiMn with thicknesses in the 0.7-3 nm range, as a probe to detect damping enhancement during magnetic phase transitions. Independent measurements of the blocking temperature with magnetometry reveal that temperature dependent shifts in the resonance peaks can also be used to measure the blocking temperature, allowing the analysis of the correlation between the N\'eel and blocking temperatures in trilayers with permalloy and antiferromagnetic layer separated by a 3 nm thick spacer layer. The thickness dependent characterization of thermal stability in antiferromagnets provides a key element for scalable and ultrafast antiferromagnetic spintronics.