Dynamical correlations and order in magic-angle twisted bilayer graphene

TL;DR

This paper uses DMFT to study electronic correlations and order in magic-angle twisted bilayer graphene, revealing how local moments, isospin ordering, and doping influence its correlated states and spectral properties.

Contribution

It introduces a detailed DMFT analysis of the THF model, elucidating the emergence of local moments, isospin order, and doping effects in twisted bilayer graphene without strain.

Findings

Local spin and valley isospin moments form around 100K.

Isospin moments order around 10K, preempting Kondo screening.

Doping causes cascades of Lifshitz transitions and spectral redistributions.

Abstract

In magic angle twisted bilayer graphene, transport, thermodynamic and spectroscopic experiments pinpoint at a competition between distinct low-energy states with and without electronic order. We use Dynamical Mean Field Theory (DMFT) on the topological heavy Fermion (THF) model of twisted bilayer graphene to investigate the emergence of electronic correlations and long-range order in the absence of strain. We contrast moment formation, Kondo screening and ordering on a temperature basis and explain the nature of emergent correlated states based on three central phenomena: (i) the formation of local spin and valley isospin moments around 100K, (ii) the ordering of the local isospin moments around 10K preempting Kondo screening, and (iii) a cascadic redistribution of charge between localized and delocalized electronic states upon doping. At integer fillings, we find that low energy spectral weight is depleted in the symmetric phase, while we find insulating states with gaps enhanced by exchange coupling in the zero-strain ordered phases. Doping away from integer filling results in distinct metallic states: a "bad metal" above the ordering temperature, where scattering off the disordered local moments suppresses electronic coherence, and a "good metal" in the ordered states with coherence of quasiparticles facilitated by isospin order. This finding reveals coherence from order as the microscopic mechanism behind the Pomeranchuk effect observed experimentally. Upon doping, there is a periodic charge reshuffling between localized and delocalized electronic orbitals leading to cascades of doping-induced Lifshitz transitions, local spectral weight redistributions and periodic variations of the electronic compressibility. Our findings provide a unified understanding of the most puzzling aspects of scanning tunneling spectroscopy, transport, and compressibility experiments.