Effect of Electron-Phonon Interactions on Three-Level QD-based Spaser: Linear and Quadratic Potentials

TL;DR

This study investigates how electron-phonon interactions, both linear and quadratic, influence the behavior and efficiency of a three-level quantum dot-based spaser, revealing effects on population inversion, phonon dynamics, and spaser intensity.

Contribution

It is the first to analyze the impact of electron-phonon interactions on QD-based spasers, considering both linear and quadratic potentials and their effects on system dynamics.

Findings

Linear interaction affects population inversion without changing spaser threshold.

Phonons exhibit decaying oscillations and steady-state behavior under continuous pumping.

Quadratic potential increases LSP number and enhances spaser spectrum intensity.

Abstract

In this article, a spaser (surface plasmon amplification by stimulated emission of radiation) system consisting of a metal nanoparticle surrounded by a large number of quantum dots (QDs) is studied. Usually, the effect of electron-phonon interaction is neglected in the spaser related literature. But some gain media, attributed by the large Raman scattering cross-section, exhibit stronger electron-phonon interaction. No such study has been performed for a QD-based spaser. Hence, it warrants investigation of the same in spaser system. In the present work, we investigate the effects of electron-phonon interaction on a three-level QD-based spaser. We consider two types of interaction potentials, linear and quadratic, and analyze their effects individually. First, we focus on the linear electron-phonon interaction that perturbs the electrons present in the excited state. This yields a periodic steady-state number of localized surface plasmon (LSP). The accompanying analytic solution reveals that the population inversion of the gain medium depends on the linear potential strength (Frohlich constant) but does not affect the threshold of spaser considerably for the given numerical parameters. In addition to the LSP, phonons may be generated during this process, the temporal dynamics of which are also detailed. Initially, the number of phonons exhibit decaying periodic oscillations, whose amplitude depends on the strength of the electron-phonon interaction. Under continuous pumping, at later times, the number of phonons reaches a steady-state value, which may find application in realization of continuous phonon nanolasers. Further, the effect of the quadratic potential is studied phenomenologically by increasing the excited-state decay rate. This results in a large number of LSP and an intense spaser spectrum.