Pressure sensitivity in non-local flow behaviour of dense hydrogel particle suspensions

TL;DR

This study demonstrates that pressure sensitivity significantly influences shear band width in dense hydrogel particle suspensions, with experimental and simulation evidence showing shear zones broaden under low confinement and narrow under compression.

Contribution

It provides the first explicit experimental validation of pressure-sensitive non-local flow models in dense hydrogel suspensions, linking microscopics to shear band localization.

Findings

Shear bands broaden at low confining stress.

Shear zones narrow with increased compression.

DEM and NGF models quantitatively match experimental data.

Abstract

Slowly sheared particulate media like sand and suspensions flow heterogeneously as they yield via narrow shear bands where most of the strain is accumulated. Understanding shear band localization from microscopics is still a major challenge. One class of so-called non-local theories identified that the width of the shearing zone should depend on the stress field. We explicitly test this picture by using a uniquely stress-sensitive suspension while probing its flow behavior in a classic geometry in which shear bands can be well-tuned: the Split-Bottom Shear Cell (SBSC). The stress-sensitive suspension is composed of mildly polydisperse soft, slippery hydrogel spheres submersed in water. We measure their flow profiles and rheology while controlling the confinement stress via hydrostatic effects and compression. We determine the average angular velocity profiles in the quasi-static flow regime using Magnetic Resonance Imaging based particle image velocimetry (MRI-PIV) and discrete element method (DEM) simulations. We explicitly match a pressure-sensitive non-local granular fluidity (NGF) model to observed flow behavior. We find that shear bands for this type of suspension become extremely broad under the low confining stresses from the almost density-matched fluid particle mixture, while collapsing to a narrow shear zone under finite, externally imposed compression levels. The DEM and NGF results match the observations quantitatively, confirming the conjectured pressure sensitivity for suspensions and its role in NGF. Our results indicate that pressure sensitivity should be part of non-local flow rules to describe slow flows of granular media.