Stimulated Brillouin scattering at 1 nm-1 wavevector by extreme ultraviolet transient gratings

TL;DR

This study demonstrates stimulated Brillouin scattering at a wavevector of approximately 1 nm-1 using extreme ultraviolet transient gratings in beta-Ga2O3, expanding the capabilities of phonon detection at short wavelengths.

Contribution

It introduces a novel EUV-based method to generate and detect high wavevector phonons via stimulated Brillouin back-scattering, bridging a gap in phonon spectroscopy techniques.

Findings

Successfully generated phonons with wavevector ~1 nm-1

Extended SBBS detection to EUV wavelengths

Provided a contact-less method for high wavevector phonon analysis

Abstract

We crossed two femtosecond extreme ultraviolet (EUV) pulses in a beta - Ga2O3 (001) single crystal to create transient gratings (TG) of light intensity with sub-100 nm spatial periodicity. The EUV TG excitation launches phonon modes, whose dynamics were revealed via the backward diffraction of a third, time-delayed, EUV probe pulse. In addition to the modes typically observed in this kind of experiment, the phase-matching condition imposed by the TG, combined with the sharp penetration depth of the EUV excitation pulses, permitted to generate and detect phonons with a wavevector tangibly larger (approximately 1 nm-1) than the EUV TG one, via stimulated Brillouin back-scattering (SBBS) of the EUV probe. While SBBS of an optical probe was reported in previous EUV TG experiments, the extension of SBBS to short wavelength radiation can be used as a contact-less experimental tool for filling the gap between the wavevector range accessible through inelastic hard X-ray and thermal neutron scattering techniques, and the one accessible through Brillouin scattering of visible and UV light.