Interfacial-antiferromagnetic-coupling driven magneto-transport properties in ferromagnetic superlattices

TL;DR

This study uses Monte-Carlo simulations to investigate how interfacial antiferromagnetic interactions in LSMO/SRO superlattices influence their magneto-transport properties, reproducing experimental phenomena and revealing the importance of carrier-driven coupling.

Contribution

It introduces a detailed model incorporating various magnetic interactions to explain complex magneto-transport phenomena in LSMO/SRO superlattices, aligning simulations with experimental observations.

Findings

Antiferromagnetic coupling causes anti-parallel alignment at low temperatures.

Reproduces positive exchange bias and inverted hysteresis loops.

Carrier-driven interactions determine metallic or insulating states depending on magnetic alignment.

Abstract

We explore the role of interfacial antiferromagnetic interaction in coupled soft and hard ferromagnetic layers to ascribe the complex variety of magneto-transport phenomena observed in $La_{0.7}Sr_{0.3}MnO_3/SrRuO_3$ (LSMO/SRO) superlattices (SLs) within a one-band double exchange model using Monte-Carlo simulations. Our calculations incorporate the magneto-crystalline anisotropy interactions and super-exchange interactions of the constituent materials, and two types of antiferromagnetic interactions between Mn and Ru ions at the interface: (i) carrier-driven and (ii) Mn-O-Ru bond super-exchange in the model Hamiltonian to investigate the properties along the hysteresis loop. We find that the antiferromagnetic coupling at the interface induces the LSMO and SRO layers to align in anti-parallel orientation at low temperatures. Our results reproduce the positive exchange bias of the minor loop and inverted hysteresis loop of LSMO/SRO SL at low temperatures as reported in experiments. In addition, conductivity calculations show that the carrier-driven antiferromagnetic coupling between the two ferromagnetic layers steers the SL towards a metallic (insulating) state when LSMO and SRO are aligned in anti-parallel (parallel) configuration, in good agreement with the experimental data. This demonstrate the necessity of carrier-driven antiferromagnetic interactions at the interface to understand the one-to-one correlation between the magnetic and transport properties observed in experiments. For high temperature, just below the ferromagnetic $T_C$ of SRO, we unveiled the unconventional three-step flipping process along the magnetic hysteresis loop. We emphasize the key role of interfacial antiferromagnetic coupling between LSMO and SRO to understand these multiple-step flipping processes along the hysteresis loop.