Field-induced bound-state condensation and spin-nematic phase in SrCu$_2$(BO$_3$)$_2$ revealed by neutron scattering up to 25.9 T

TL;DR

This study uses high-field neutron scattering and advanced calculations to reveal a spin-nematic phase in SrCu$_2$(BO$_3$)$_2$, characterized by bound-state condensation and unconventional excitations, expanding understanding of quantum magnetic states.

Contribution

First high-field neutron scattering measurements combined with MPS calculations to identify a spin-nematic phase in SrCu$_2$(BO$_3$)$_2$, demonstrating bound-state condensation under extreme conditions.

Findings

Observation of a spin-nematic phase induced by high magnetic fields.

Detection of multiple multi-magnon bound states and novel excitations.

Persistence of a one-magnon spin gap indicating unconventional order.

Abstract

Bose-Einstein condensation (BEC) underpins exotic forms of order ranging from superconductivity to superfluid 4 He. In quantum magnetic materials, ordered phases induced by an applied magnetic field can be described as the BEC of magnon excitations. With sufficiently strong magnetic frustration, exemplified by the system SrCu$_2$(BO$_3$)$_2$ , no clear magnon BEC is observed and the complex spectrum of multi-magnon bound states may allow a different type of condensation, but the high fields required to probe this physics have remained a barrier to detailed investigation. Here we exploit the first purpose-built high-field neutron scattering facility to measure the spin excitations of SrCu$_2$(BO$_3$)$_2$ up to 25.9 T and use cylinder matrix-product-states (MPS) calculations to reproduce the experimental spectra with high accuracy. Multiple unconventional features point to a condensation of $S = 2$ bound states into a spin-nematic phase, including the gradients of the one-magnon branches, the presence of many novel composite two- and three-triplon excitations and the persistence of a one-magnon spin gap. This gap reflects a direct analogy with superconductivity, suggesting that the spin-nematic phase in SrCu$_2$(BO$_3$)$_2$ is best understood as a condensate of bosonic Cooper pairs. Our results underline the wealth of unconventional states yet to be found in frustrated quantum magnetic materials under extreme conditions.