Scaling behaviour of the helical and skyrmion phases of Cu2OSeO3 determined by single crystal small angle neutron scattering

TL;DR

This study maps the phase diagram of Cu2OSeO3, revealing how skyrmion and helical magnetic phases depend on temperature, magnetic field, and crystal orientation, providing insights crucial for future skyrmion-based technologies.

Contribution

It presents detailed phase diagrams and scaling behavior of skyrmion and helical phases in Cu2OSeO3, including effects of crystal orientation and cooling procedures, advancing understanding of skyrmion formation and control.

Findings

Determined stability ranges of magnetic phases in Cu2OSeO3.

Analyzed skyrmion and helical phase scaling and packing density.

Identified effects of crystal orientation and cooling on skyrmion stability.

Abstract

Skyrmions are topologically protected quantum objects at the nanometre scale. They form perpendicular to an applied magnetic field at a certain temperature and arrange themselves in a typically hexagonal lattice. Using small angle neutron scattering we have determined the magnetic field versus temperature phase diagrams of the stability range of the different magnetic phases, the helical as well as the skyrmion phases in the multiferroic skyrmion material Cu$_2$OSeO$_3$. Therefore, a single crystal was mounted in different crystal orientations, i.e. unoriented and with the crystallographic $\langle1 1 0\rangle$ and $\langle1 0 0\rangle$ axis aligned parallel to the magnetic field. Furthermore, different cooling procedures were tested, cooling from the paramagnetic phase at zero magnetic field and field cooling through the skyrmion phase where metastable skyrmions are nucleated. From this, not only were the stability ranges of both the helical and skyrmion phases in this multiferroic skyrmion material determined, but the length of the spin helix and the skyrmion distances at different conditions was also determined through detailed analysis of the positions of the observed Bragg peaks. The obtained data provide valuable information about the scaling of the skyrmion distances and therefore their packing density. The knowledge about this tunability will serve as an important input for the theoretical understanding of the formation of skyrmions. Concerning technological applications, for example as high-density data storage devices in information technology, the temperature and magnetic field dependence of the packing density of skyrmions is of critical importance for their design. Therefore, the obtained knowledge is an essential input for future skyrmionics applications in high-density data storage, in low-energy spintronics or in skyrmionics quantum computation.