New perspectives on spectroscopic factor quenching from reactions
Chlo\"e Hebborn, Filomena M. Nunes, Amy E. Lovell

TL;DR
This study reconciles discrepancies in spectroscopic factor quenching by analyzing transfer and knockout reactions with Bayesian uncertainty quantification, revealing a consistent, small asymmetry dependence of single-particle strengths in nuclei.
Contribution
It provides the first consistent Bayesian analysis of transfer and knockout data, quantifying uncertainties and resolving a long-standing puzzle in nuclear spectroscopic strengths.
Findings
Transfer and knockout spectroscopic strengths agree within uncertainties.
Both probes indicate a small asymmetry dependence of single-particle strengths.
Uncertainties are larger than previous estimates, setting a lower bound.
Abstract
The evolution of single-particle strengths as the neutron-to-proton asymmetry changes informs us of the importance of short- and long-range correlations in nuclei and has therefore been extensively studied for the last two decades. Surprisingly, the strong asymmetry dependence of these strengths and their extreme values for highly-asymmetric nuclei inferred from knockout reaction measurements on a target nucleus are not consistent with what is extracted from electron-induced, transfer, and quasi-free reaction data, constituting a two-decade old puzzle. This work presents the first consistent analysis of one-nucleon transfer and one-nucleon knockout data, in which theoretical uncertainties associated with the nucleon-nucleus effective interactions considered in the reaction models are quantified using a Bayesian analysis. Our results demonstrate that, taking into account these…
| [MeV] | ||||
|---|---|---|---|---|
| 32Ar | 21.60 | 5/2+ | 05/2 | |
| 34Ar | 17.07 | 0+ | 11/2 | |
| 36Ar | 15.26 | 0+ | 3/2+ | |
| 46Ar | 8.07 | 0+ |
| [mb] | [mb] | [mb] | [mb] | |
|---|---|---|---|---|
| 32Ar | 10.4 | 2.7 | 6.3 | |
| 34Ar | 4.7 | 12.8 | 4.2 | 8.6 |
| 46Ar | 61 | 13.4 | 4.2 | 9.2 |
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Taxonomy
TopicsNuclear physics research studies · Advanced Chemical Physics Studies · Advanced NMR Techniques and Applications
New perspectives on spectroscopic factor quenching from reactions
C. Hebborn
Facility for Rare Isotope Beams, Michigan State University, East Lansing, Michigan 48824, USA
Lawrence Livermore National Laboratory, P.O. Box 808, L-414, Livermore, California 94551, USA
F. M. Nunes
Facility for Rare Isotope Beams, Michigan State University, East Lansing, Michigan 48824, USA
Department of Physics and Astronomy, Michigan State University, East Lansing, Michigan 48824, USA
A. E. Lovell
Theoretical Division, Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA
Abstract
The evolution of single-particle strengths as the neutron-to-proton asymmetry changes informs us of the importance of short- and long-range correlations in nuclei and has therefore been extensively studied for the last two decades. Surprisingly, the strong asymmetry dependence of these strengths and their extreme values for highly-asymmetric nuclei inferred from knockout reaction measurements on a target nucleus are not consistent with what is extracted from electron-induced, transfer, and quasi-free reaction data, constituting a two-decade old puzzle. This work presents the first consistent analysis of one-nucleon transfer and one-nucleon knockout data, in which theoretical uncertainties associated with the nucleon-nucleus effective interactions considered in the reaction models are quantified using a Bayesian analysis. Our results demonstrate that, taking into account these uncertainties, the spectroscopic strengths of loosely-bound nucleons extracted from both probes agree with each other and, although there are still discrepancies for deeply-bound nucleons, the slope of the asymmetry dependence of the single-particle strengths inferred from transfer and knockout reactions are consistent within . Both probes are consistent with a small asymmetry dependence of these strengths. The uncertainties obtained in this work represent a lower bound and are already significantly larger than the original estimates.
††preprint: LLNL-JRNL-845215, LA-UR-23-21722
Introduction: Systematic studies of nuclei along isotopic chains have revealed unexpected trends that challenge our understanding of nuclear structure Tanihata et al. (2013); Otsuka et al. (2020); Nunes (2021). While energy spectra hold an important component of this complex many-body puzzle, reaction studies since the 50s have been extracting information on the composition of the nuclear wavefunction itself, and in particular the distribution of strength across various nuclear orbitals. This is expressed in terms of a spectroscopic factor (SF), proportional to the probability that the system will be found in a particular configuration. These SFs are reduced compared to the independent particle model (IPM), due to long-range correlations (LRC), associated mainly with pairing and deformation effects, and short-range correlations (SRC). The evolution of this shell structure away from stability therefore provides unique insights on correlations in nuclei and on the fundamental nuclear force Otsuka et al. (2020); Aumann et al. (2021). Moreover, because SRCs influence the equation of state Hen et al. (2015), are connected with the quark momentum distributions in nucleons bound inside nuclei Weinstein et al. (2011), and affect lepton-nucleus interactions Gallagher et al. (2011), an accurate understanding of SRCs will impact astrophysics, particle physics and neutrino physics.
The importance of these correlations in nuclei is quantified by comparing SFs extracted from experimental nucleon-removal data and theoretical predictions Aumann et al. (2021). For two decades, nuclear physicists have grappled with the asymmetry dependence of the ratio between the SF extracted from experiment and that predicted by the nuclear shell model. The now famous asymmetry plot showing as a function of the difference between neutron and proton separations energies () has caused significant debate Aumann et al. (2021). The asymmetry dependence of found in the analysis of one-nucleon knockout reactions on a 9Be or 12C targets–often referred simply as knockout reactions–Gade et al. (2008); Tostevin and Gade (2014, 2021) is not consistent with that found using other probes, namely for electron-induced Kramer et al. (2001), quasi-free Gómez-Ramos and Moro (2018) and transfer reactions Tsang et al. (2009); Lee et al. (2006); Kay et al. (2013) (see the recent review Ref. Aumann et al. (2021) for a full status). For the last two decades, many studies have attempted to understand the source of this inconsistency. Our work adds to these studies, although it brings a novel perspective.
SFs are model dependent Duguet et al. (2015); Tropiano et al. (2021); their extraction from experimental data require both a reaction model and a structure model. The analysis of knockout reactions makes use of the eikonal reaction theory as well as large-scale shell-model calculations. To understand the asymmetry dependence of associated with knockout observables, the validity of the shell-model SFs and the eikonal model have been thoroughly analyzed, e.g. Refs. Jensen et al. (2011); Barbieri (2009); Cipollone et al. (2015); Wylie et al. (2021); Atkinson and Dickhoff (2019); Paschalis et al. (2020) discuss the importance of SRCs and LRCs for structure predictions and Refs. Flavigny et al. (2012); Louchart et al. (2011); Gómez-Ramos et al. (2021); Lei and Bonaccorso (2021); Bertulani and McVoy (1992); Hebborn and Capel (2019); Capel et al. (2008) address the validity of the eikonal approximation. Similarly, many studies tested the validity of the theories used in the transfer analyses Nunes et al. (2011); Chazono et al. (2017); Nunes and Deltuva (2011); Upadhyay et al. (2012), including benchmarks of the reaction models.
Given that SFs are not observables, a degree of caution needs to be taken in interpreting the results. When using different probes, it is essential to make the same assumptions so the conclusions are both comparable and reliable. Equally necessary is a good understanding of the theoretical uncertainties without which any disagreement between results is rendered meaningless. One earlier study did attempt to quantify the uncertainties associated with the reaction theory used in the transfer Nunes et al. (2011) however those estimates were obtained without a rigorous statistical analysis.
Although in the majority of cases, the plots contain only statistical errors from the experimental data, we understand there are significant uncertainties attributed to the reaction models themselves. Most noteworthy are the uncertainties associated with the phenomenological fits of the effective interactions used, the so-called optical potentials Hebborn et al. (2023a). Bayesian analyses of elastic scattering has led to the understanding that uncertainties associated with the optical potentials are larger than previously estimated Lovell et al. (2020); Lovell and Nunes (2018); Catacora-Rios et al. (2023); Hebborn et al. (2023b). This work offers the first consistent analysis of knockout and transfer reaction data on three different Ar isotopes using Bayesian statistics to quantify the theoretical uncertainties associated with the nucleon-nucleus optical potentials.
Methodology: We first reanalyze transfer data for the 34,36,46Ar33,35,45Ar(g.s.) reactions at MeV Lee et al. (2010), using the Adiabatic Wave Approximation (ADWA) Johnson and Tandy (1974), and take as input the nucleon- and nucleon- interactions at the beam energy and at half the deuteron energy for the incoming and outgoing channels, respectively. The nucleon-Ar optical potential parameters are directly sampled111We sampled the multivariate Gaussian posterior distributions generated by the python script provided in the Supplemental Material of Ref. Pruitt et al. (2023) from the recent global parameterization KDUQ Pruitt et al. (2023) from which we compute the credible intervals for the transfer angular distributions using the code nlat Titus et al. (2016).
We reanalyze 32ArBe31Ar(g.s.) at MeV Gade et al. (2004a) and 34,46ArBe33,45Ar(g.s.) at MeV Gade et al. (2004b, 2005), using the eikonal method Glauber (1959); Hussein and McVoy (1985); Hansen and Tostevin (2003); Capel et al. (2008), and we quantify the uncertainties arising from the -9Be target interaction only. Because KDUQ is not appropriate for light targets, we follow the work done in Ref. Hebborn et al. (2023b), and instead we generate mock elastic angular distributions with a realistic potential Weppner (2018). We assign to these mock data an error of , which is common for elastic-scattering experiments with stable beams. Parameter posterior distributions are obtained from the Bayesian analysis of the -9Be target elastic scattering and are propagated to obtain credible intervals for the knockout momentum distributions. For the core-9Be interaction, we use the optical limit with the parameters of Ref. Abu-Ibrahim et al. (2008) and the density of approximated by two-parameter Fermi distributions Chamon et al. (2002). We do not include the uncertainties associated with the core-9Be interaction as there are no elastic-scattering data on these systems or realistic potential to generate mock data and it has been shown that the uncertainties arising from this interaction are less significant Hebborn et al. (2023b). In both the transfer and knockout calculations, we do not include the spin-orbit force for convenience, since we expect it to have a negligible effect.
Critical to both reaction calculations are the structure input: the exact same description is used for the single-particle structure of the isotopes involved. We use a Wood-Saxon potential with a radius of fm with fm and diffuseness of fm222We have verified that our conclusions do not change when using a different geometry ( fm and fm with fm) for this Woods-Saxon potential. and we fit its depth to the neutron separation energy. Details concerning the relevant single-particle states used in the transfer and knockout calculations are given in Table 1.
Results: The transfer angular distributions are shown in Fig. 1: the normalized 68% (dark shaded blue) and 95% (light shaded blue) credible intervals are compared to the data reported in Ref. Lee et al. (2010). The shape of the predicted transfer angular distributions are in good agreement with experiment, corroborating the assumptions made in ADWA.
The results for parallel-momentum distributions following knockout are shown in Fig. 2: the normalized 68% (dark shaded salmon) and 95% (light shaded salmon) credible intervals are compared to the data reported in Refs. Gade et al. (2004a, b, 2005). In general, the experimental distributions are well reproduced by the eikonal model, except for the 46Ar case, which exhibits a highly-asymmetric distribution. As discussed in Ref. Gade et al. (2005), this low-momentum tail is likely due to additional, dissipative mechanisms acting in the final state of the reaction products, which are not included in the eikonal approximation. We will discuss how this impacts the extracted SF later.
The parallel-momentum distributions are numerically integrated to obtain the total knockout cross sections shown in Table 2: the experimental total cross sections (, 2nd column) are listed along with the theoretical ones, namely the diffractive-breakup contributions (, 4th column), the stripping contributions333The diffractive-breakup contribution corresponds to the reaction channel in which both the core and the neutron survive the collision, and the stripping to the channel in which the neutron is absorbed by the target. (, 5th column) and the total predicted single-particle cross sections (, 3rd column). It is clear that the errors on the theoretical total knockout cross section are also mostly defined by the uncertainties in the stripping component. This feature is expected for the removal of well-bound neutrons (all cases considered in this work have neutron separation energies MeV) which makes the reaction process more sensitive to the details of the optical potentials Hebborn et al. (2023b).
We now consider the extraction of the SFs. For transfer, we follow a similar procedure as in Ref. Nunes et al. (2011): we extract the SF by adjusting the angular distributions to the data points around the peak. The corresponding SFs and their uncertainties are displayed in the 2nd column of Table 3, along with the () errors. Our SFtran are consistent with those extracted in Ref. Nunes et al. (2011) (3rd column) although they exhibit larger errors. The relative uncertainty in SFtran increases with the binding energy of the projectile, similarly to what was observed in knockout observables Hebborn et al. (2023b). For knockout, we sample both the total cross section posterior distribution predicted by theory and the corresponding experimental total cross sections, assuming a normal distribution. We then extract the distribution of the SFs by taking the ratio of the experimental samples with the theoretical ones. The corresponding SFko, shown in the 4th column of Table 3, are consistent with the ones extracted in the original analyses (5th column) Gade et al. (2004a, b, 2005). However, the original uncertainties for SFko are much smaller than those we obtained here, just as was found in the transfer case. Note that the SFs extracted from knockout data on 46Ar (34Ar) are consistent with the ones extracted from the transfer data within ().
To obtain the ratio , we use previously published large-scale shell model calculations444These spectroscopic factors include the center-of-mass correction with the major oscillator quantum number Dieperink and Forest (1974); Hansen and Tostevin (2003).: SF for 32Ar Gade et al. (2004a), and SF for 34,36,46Ar Lee et al. (2010). No uncertainties have been estimated for these predictions. As noted in earlier analyses Gade et al. (2008); Tostevin and Gade (2014, 2021), the shell-model SFs are significantly larger than the SFs extracted from the knockout of deeply-bound nuclei, e.g. 32,34Ar, but are in agreement with those extracted from transfer. The fact that for some reactions, we have SFSFSM and SFSFSM, highlights again that SFs are model construct. In theoretical structure calculations, SFs are normalized to ensure the nucleon number conservation. However, when extracted from experimental data, SFs do not ensure the nucleon number conservation as the theoretical model used to analyze the data inconsistently treats structure and reaction properties.
Fig. 3 contains the asymmetry dependence of using transfer (blue bars) and knockout (red bars) data. The thick bars represented and the thin bars represent , both obtained from the credible intervals on the SFs reported in Table 3. We must point out that the results for obtained for the three discrete values of are not necessarily consistent with a linear dependence, either for transfer or for knockout. Nevertheless, for the sake of comparison with previous studies, we fit to , for each reaction case, transfer or knockout, taking into account the uncertainty (blue and salmon shaded bands). The slope obtained for transfer () is consistent with the slope obtained for knockout (), within uncertainties, even though there are significant differences in the values of the intercept ( for transfer and for knockout). Our extracted slope for knockout is consistent with that extracted previously ( Tostevin and Gade (2021)) however now we include the uncertainty coming from both the optical potentials in the theoretical analysis and the experimental errors.
Discussion: An optical model dependence on the overall normalization of the extracted SFs might be expected, but we have verified that the slope obtained is not dependent on the choice of the optical potential. When repeating the knockout analysis using KDUQ, the same parameterization used in the transfer analysis, we obtained a slope of (shown in the Supplemental Material, which includes Ref. Koning and Delaroche (2003)). In addition to transfer and knockout, and reactions have also been studied in this context Gómez-Ramos and Moro (2018). Although to make a meaningful comparison, similar uncertainty analysis for those reaction channels needs to be done, our results do not seem inconsistent with Ref. Gómez-Ramos and Moro (2018).
As pointed out in Ref. Gómez-Ramos and Moro (2018), the asymmetry dependence extracted can change slightly when using shell-model predictions with different residual interactions and/or model spaces, or even when using different model assumptions for the geometry of the single-particle wave function. Yet, there will be no significant change on the relative uncertainties due to the optical potentials. To remove any possible dependence on the shell model and to facilitate a future comparison with results obtained from measurements, we also provide the asymmetry plot when is extracted using the IPM occupation numbers in Supplemental Material (the ratio deduced from the data Kramer et al. (2001) relies on the IPM). The results for using IPM do not seem inconsistent with those of Ref. Kramer et al. (2001), however a study of the uncertainty in that reaction probe remains to be completed.
One must keep in mind that the uncertainties here presented are only a lower bound. First, we did not include the parametric uncertainties associated with the description of the single-particle state Catacora-Rios et al. (2023) even though we did use the exact same model in both analyses. For this reason, we expect these uncertainties to have no impact on our conclusions. Moreover, we did not quantify the uncertainties associated with the core-target potentials, used to compute knockout cross sections. More intricate is the quantification of model uncertainties. The reaction models used to interpret the measurements have approximations and therefore a complete analysis should include the errors associated with them. Although the inclusion of model uncertainties is beyond the scope of this work, there are plans to tackle this problem in the near future and it is important to identify the theory approximation in the models that are likely to be more relevant. Next, we briefly discuss this aspect.
In transfer reactions, ADWA has been benchmarked against Faddeev calculations, solving the three-body problem exactly Nunes et al. (2011): at MeV the differences are only significant for the 36Ar case but a more rigorous quantification is desirable. In knockout, the measured momentum distributions exhibit an asymmetry for 46Ar that the model does not predict. The interpretation of the knockout data relies on the eikonal model, which contains two approximations: the adiabatic approximation and a core-spectator approximation. The adiabatic approximation violates energy conservation and is the cause for the symmetric parallel-momentum distributions (as seen in Fig. 2(c)). Improved models which do conserve energy are able to describe the distributions (e.g., Ref. Flavigny et al. (2012)). It has been shown that the integrated cross sections produced in such models agree with those from the eikonal model, proving that this aspect does not have a strong impact on the extracted SFs Gómez-Ramos et al. (2021). The second approximation, the core-spectator approximation, assumes that the core degrees of freedom are “frozen” during the collision process. However, dissipative mechanisms associated with the removal of the nucleon tend to decrease the predicted cross sections Louchart et al. (2011), an effect that is more important the more bound the system is. We expect that the extracted SFs obtained from knockout data when including these dissipative effects would be larger for nuclei with large , which could explain part of the apparent discrepancies between transfer and knockout predictions in Fig. 3. Unfortunately, accounting for these dissipative effects is not trivial and requires updated reaction frameworks. Initial studies in the reaction theory community are moving in this direction Gómez-Ramos et al. (2022); Hebborn and Potel (2023) but more work is needed, including the coupling of the new frameworks with a Bayesian analysis.
Conclusions: In summary, we reanalyze a set of transfer and knockout data using a Bayesian framework to quantify the theoretical uncertainties due to the optical potentials, known to be one of the leading sources of uncertainties in reaction models. In the past, optical potentials uncertainties were estimated naïvely by comparing the results with two arbitrary parameterizations Nunes et al. (2011). This work demonstrates that those original estimates produce uncertainties that are significantly underestimated. Most importantly, our results show that, when the optical potential uncertainties are included in a robust statistical approach, transfer and knockout reactions lead to a consistent picture for the removal of a loosely-bound nucleon and both probes are consistent with a small asymmetry dependence of SFs. This work also shows that there is still some tension between the strengths extracted from transfer and knockout data on deeply-bound nuclei as they only agree within . These tensions come likely from model uncertainties that have not been quantified in this analysis, and will be the focus of future works. Even though theoretical uncertainties need to be quantified in the analysis of , and data to make a meaningful comparison between these probes and the present work, the slopes that we extract here do not seem inconsistent with previous analyses of those data Gómez-Ramos and Moro (2018); Kramer et al. (2001).
Finally, it is also clear that to infer accurate and precise information from reaction data, optical potentials need to be better constrained. Of particular relevance are their imaginary strengths simulating the loss of flux from the elastic channel due to open reaction channels and their isospin dependence which drives the extrapolation of these interactions to unstable nuclei. To improve these phenomenological interactions, one can enforce the dispersion conditions, relating the real and imaginary parts of the interaction in the appropriate manner Dickhoff and Charity (2019), and consider other type of reaction data, e.g., charge-exchange, to constrain their isospin dependence. These dispersive potentials provide a consistent framework to describe the structure and reaction properties. The extension of the Bayesian framework in this direction is being pursued.
Acknowledgements.
*Acknowledgments. * C. H. would like to thank L. Moschini for sharing her code computing the nuclear eikonal phase within the optical limit approximation and A. Gade for sharing the knockout data on 34Ar. Valuable discussions with T. R. Whitehead are acknowledged. C. H. would like to thank K. Kravvaris, G. Potel and C. D. Pruitt for interesting discussions. C. H. acknowledges the support of the U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under the FRIB Theory Alliance award no. DE-SC0013617 and under Work Proposal no. SCW0498. A. E. L. acknowledges the support of the Laboratory Directed Research and Development program of Los Alamos National Laboratory. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344 and by Los Alamos National Laboratory under Contract 89233218CNA000001. F. M. N. acknowledges the support of the U.S. Department of Energy grant DE-SC0021422. This work relied on iCER and the High Performance Computing Center at Michigan State University for computational resources.
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