Generation, dynamics, and correlations of the fission fragments' angular momenta

TL;DR

This paper presents a time-dependent collective Hamiltonian model to better understand the generation and correlation of angular momenta in fission fragments, aligning with experimental data and revealing new insights into fragment dynamics.

Contribution

A novel time-dependent collective Hamiltonian model is developed to analyze angular momentum generation and correlations in fission fragments, incorporating quantum uncertainty and fragment deformations.

Findings

Model accounts for a large part of experimental angular momentum data.

Fragment angular momenta are mainly perpendicular to the fission axis.

Fragment angular momenta are nearly uncorrelated, with some positive correlation observed.

Abstract

The generation of angular momentum in fissioning nuclei is not well understood. The predictions of different models disagree, particularly concerning the correlation between the fragments' angular momenta. In this article, a time-dependent collective Hamiltonian model is proposed to treat the generation of the angular momentum in the fission fragments due to the quantum uncertainty principle as well as the dynamics of the collective wave function during and after scission. The model is constructed in the framework of the frozen Hartree-Fock approximation using a Skyrme energy functional to extract deformations of the fission fragments as well as the interactions in a derived collective Hamiltonian. The fission reactions studied are $^{240}$Pu $\rightarrow$ $^{132}$Sn+$^{108}$Ru and $^{240}$Pu $\rightarrow$ $^{144}$Ba+$^{96}$Sr. The model can account for a large part of the angular momentum found in experimental data. The orientation of the angular momentum of each fragment is found to be mainly in the plane perpendicular to the fission axis, in agreement with the experiment. The magnitudes of the angular momenta in the two fragments are nearly uncorrelated, in agreement with the recent experimental data of Wilson et al., Nature (London) 590, 566 (2021). Some of the conclusions of the traditional collective vibration model are supported by the present model but some are not. Surprisingly, it is found that the angular momenta of the fragments are slightly correlated positively as in a wriggling mode. It is also found that the presence of an octupole deformation in a fragment can significantly increase the generated angular momentum.