Laser-assisted Fano resonance: attosecond quantum control and dynamical imaging

TL;DR

This paper introduces a laser-assisted Fano resonance technique that enables attosecond control and imaging of electron wave packets, allowing measurement of photoionization time delays with unprecedented resolution.

Contribution

It presents the concept of laser-assisted Fano resonance and demonstrates its application in real-time imaging and control of electron dynamics at attosecond scales.

Findings

Active control of Fano lineshape on attosecond timescale

Direct imaging of resonant electron wave packets

Measurement of resonant photoionization time delay

Abstract

A Fano resonance arises from the pathway interference between discrete and continuum states, playing a fundamental role in many branches of physics, chemistry and material science. Here, we introduce the concept of a laser-assisted Fano resonance, created from two interferometric pathways that are coupled together by an additional laser field, which introduces a controllable phase delay between them and results in a generalized Fano lineshape that can be actively controlled on the {\it attosecond} time scale. Based on our experimental results of unprecedented resolution, we dynamically image a resonant electron wave packet during its evolution directly in the time domain, extracting both the amplitude and the phase, which allows for the measurement of the {\it resonant} photoionization time delay. Ab-initio calculations and simulations employing a physically transparent two-level model agree with our experimental results, laying the groundwork for extending our concepts into attosecond quantum control of complex systems.