Inhomogeneous superconductivity onset in FeSe studied by transport properties

TL;DR

This study investigates the onset of inhomogeneous superconductivity in FeSe by measuring transport properties across different sample thicknesses, revealing increased $T_c$ in thinner samples and providing a method to estimate domain aspect ratios.

Contribution

The paper introduces a new method to estimate the aspect ratio of superconducting domains from $T_c$ anisotropy and extends conductivity models to anisotropic, elongated domains in FeSe.

Findings

$T_c$ increases from 8 K to 12 K as sample thickness decreases.

A method to estimate SC domain aspect ratio from $T_c$ anisotropy.

Analytical formulas for conductivity in elongated, anisotropic SC domains.

Abstract

Heterogeneous superconductivity onset is a common phenomenon in high-$T_c$ superconductors of both the cuprate and iron-based families. It is manifested by a fairly wide transition from the metallic to zero-resistance state. Usually, in these strongly anisotropic materials, superconductivity (SC) first appears as isolated domains. This leads to anisotropic excess conductivity above $T_c$, and the transport measurements provide valuable information about the SC domain structure deep within the sample. In bulk samples, this anisotropic SC onset gives an approximate average shape of SC grains, while in thin samples it also indicates the average size of SC grains. In this work, both interlayer and intralayer resistivity are measured as a function of temperature in FeSe samples of various thickness. To measure the interlayer resistivity, FeSe mesa structures oriented across the layers were fabricated using FIB. As the sample thickness decreases, a significant increase in superconducting transition temperature $T_c$ is observed : $T_c$ raises from 8 K in bulk material to 12 K in microbridges of thickness $\sim 40$ nm. We apply analytical and numerical calculations to analyze these and earlier data and find the aspect ratio and size of the SC domains in FeSe consistent with our resistivity and diamagnetic response measurements. We propose a simple and fairly accurate method for estimating the aspect ratio of SC domains from $T_c$ anisotropy in samples of various small thickness. The relationship between nematic and superconducting domains in FeSe is discussed. We also generalize the analytical formulas for conductivity in heterogeneous anisotropic superconductors to the case of elongated SC domains of two perpendicular orientations with equal volume fractions, corresponding to the nematic domain structure in various Fe-based superconductors.