Scanning tunneling microscopy study of hidden phases in atomically thin 1T-TaS$_2$

TL;DR

This study uses scanning tunneling microscopy to uncover hidden stripe phases in atomically thin 1T-TaS$_2$, revealing their coexistence with charge-density waves and potential implications for electronic phenomena.

Contribution

It demonstrates electrically induced and spontaneously emerging hidden stripe phases in atomically thin 1T-TaS$_2$, advancing understanding of phase transitions in low-dimensional materials.

Findings

Hidden stripe phase can be electrically induced at room temperature.

The hidden stripe phase coexists with nearly commensurate charge-density-wave phase.

Spontaneous emergence of stripe phase observed on tiny flakes without electric excitation.

Abstract

Lower thermal stability due to thinning often leads to unprecedented hidden phases in low-dimensional materials. Such hidden phases can coexist or compete with preexisting electronic phases. We investigate hidden phases observed in atomically thin (6-8 layers) 1T-TaS$_2$ with scanning tunneling microscopy. First, we can electrically induce a hidden stripe phase at room temperature. Such a uniaxial stripe phase has three equivalent orientations by breaking three-fold symmetry of 1T-TaS$_2$. We also reveal that the hidden stripe phase coexists with nearly commensurate charge-density-wave phase. Next, we observe that the emergent stripe phase spontaneously appears without any electric excitation on a tiny flake ($160\times80$ nm$^2$). Our findings may provide a plausible explanation for the previously observed phase transition and two-fold optical response in thin 1T-TaS$_2$ devices at room temperature. Furthermore, the hidden stripe phase would be crucial to understand exotic CDW-related phenomena in 1T-TaS$_2$ for potential applications.